Law Simon, Panwar Preety, Li Jody, Aguda Adeleke H, Jamroz Andrew, Guido Rafael V C, Brömme Dieter
Department of Biochemistry and Molecular Biology, Faculty of Medicine, University of British Columbia, Vancouver, British Columbia, Canada.
Centre for Blood Research, University of British Columbia, Vancouver, British Columbia, Canada.
PLoS One. 2017 Oct 31;12(10):e0186869. doi: 10.1371/journal.pone.0186869. eCollection 2017.
Cathepsin K (CatK) is a cysteine protease that plays an important role in mammalian intra- and extracellular protein turnover and is known for its unique and potent collagenase activity. Through studies on the mechanism of its collagenase activity, selective ectosteric sites were identified that are remote from the active site. Inhibitors targeting these ectosteric sites are collagenase selective and do not interfere with other proteolytic activities of the enzyme. Potential ectosteric inhibitors were identified using a computational approach to screen the druggable subset of and the entire 281,987 compounds comprising Chemical Repository library of the National Cancer Institute-Developmental Therapeutics Program (NCI-DTP). Compounds were scored based on their affinity for the ectosteric site. Here we compared the scores of three individual molecular docking methods with that of a composite score of all three methods together. The composite docking method was up to five-fold more effective at identifying potent collagenase inhibitors (IC50 < 20 μM) than the individual methods. Of 160 top compounds tested in enzymatic assays, 28 compounds revealed blocking of the collagenase activity of CatK at 100 μM. Two compounds exhibited IC50 values below 5 μM corresponding to a molar protease:inhibitor concentration of <1:12. Both compounds were subsequently tested in osteoclast bone resorption assays where the most potent inhibitor, 10-[2-[bis(2-hydroxyethyl)amino]ethyl]-7,8-diethylbenzo[g]pteridine-2,4-dione, (NSC-374902), displayed an inhibition of bone resorption with an IC50-value of approximately 300 nM and no cell toxicity effects.
组织蛋白酶K(CatK)是一种半胱氨酸蛋白酶,在哺乳动物细胞内和细胞外蛋白质周转中起重要作用,并以其独特而强大的胶原酶活性而闻名。通过对其胶原酶活性机制的研究,确定了远离活性位点的选择性别构位点。靶向这些别构位点的抑制剂具有胶原酶选择性,不会干扰该酶的其他蛋白水解活性。使用计算方法筛选了美国国立癌症研究所-发展治疗项目(NCI-DTP)化学储存库库中281,987种化合物的可药用子集和全部化合物,以确定潜在的别构抑制剂。根据化合物对别构位点的亲和力进行评分。在这里,我们将三种单独的分子对接方法的评分与这三种方法的综合评分进行了比较。综合对接方法在识别强效胶原酶抑制剂(IC50 < 20 μM)方面比单独的方法有效多达五倍。在酶促试验中测试的160种顶级化合物中,有28种化合物在100 μM时显示出对CatK胶原酶活性的阻断作用。两种化合物的IC50值低于5 μM,对应的蛋白酶:抑制剂摩尔浓度<1:12。随后在破骨细胞骨吸收试验中对这两种化合物进行了测试,其中最有效的抑制剂10-[2-[双(2-羟乙基)氨基]乙基]-7,8-二乙基苯并[g]蝶啶-2,4-二酮(NSC-374902)显示出对骨吸收的抑制作用。IC50值约为300 nM,且无细胞毒性作用。