Jet Propulsion Laboratory, California Institute for Technology, Pasadena, 91109, CA, USA.
Institute for Marine and Atmospheric Research Utrecht, Utrecht University, Utrecht, The Netherlands.
Nat Commun. 2017 Dec 20;8(1):2227. doi: 10.1038/s41467-017-02246-0.
Several viable but conflicting explanations have been proposed to explain the recent ~8 p.p.b. per year increase in atmospheric methane after 2006, equivalent to net emissions increase of ~25 Tg CH per year. A concurrent increase in atmospheric ethane implicates a fossil source; a concurrent decrease in the heavy isotope content of methane points toward a biogenic source, while other studies propose a decrease in the chemical sink (OH). Here we show that biomass burning emissions of methane decreased by 3.7 (±1.4) Tg CH per year from the 2001-2007 to the 2008-2014 time periods using satellite measurements of CO and CH, nearly twice the decrease expected from prior estimates. After updating both the total and isotopic budgets for atmospheric methane with these revised biomass burning emissions (and assuming no change to the chemical sink), we find that fossil fuels contribute between 12-19 Tg CH per year to the recent atmospheric methane increase, thus reconciling the isotopic- and ethane-based results.
已经提出了几种可行但相互矛盾的解释来解释 2006 年后大气甲烷每年约增加 8 个 ppb 的现象,相当于每年净排放增加约 25 太克甲烷。大气乙烷的同时增加暗示了化石源;甲烷重同位素含量的同时下降表明其源自生物源,而其他研究则提出化学汇(OH)减少。在这里,我们使用 CO 和 CH 的卫星测量结果表明,从 2001-2007 年到 2008-2014 年,甲烷的生物质燃烧排放量每年减少了 3.7(±1.4)太克甲烷,几乎是先前估计值的两倍。在更新了大气甲烷的总预算和同位素预算(并假设化学汇没有变化)后,我们发现化石燃料每年向大气甲烷增加贡献 12-19 太克甲烷,从而调和了基于同位素和乙烷的结果。