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从硅烯单层到Ag(111)上的薄硅膜的转变:实验数据与蒙特卡罗模拟的比较

Transition from silicene monolayer to thin Si films on Ag(111): comparison between experimental data and Monte Carlo simulation.

作者信息

Curcella Alberto, Bernard Romain, Borensztein Yves, Pandolfi Silvia, Prévot Geoffroy

机构信息

Sorbonne Universités, UPMC Univ Paris 06, CNRS-UMR 7588, Institut des NanoSciences de Paris, F-75005, Paris, France.

出版信息

Beilstein J Nanotechnol. 2018 Jan 5;9:48-56. doi: 10.3762/bjnano.9.7. eCollection 2018.

Abstract

Scanning tunneling microscopy (STM), Auger electron spectroscopy (AES) and low energy electron diffraction have been used to follow the growth of Si films on Ag(111) at various temperatures. Using a simple growth model, we have simulated the distribution of film thickness as a function of coverage during evaporation, for the different temperatures. In the temperature regime where multilayer silicene has been claimed to form (470-500 K), a good agreement is found with AES intensity variations and STM measurements within a Ag surfactant mediated growth, whereas a model with multilayer silicene growth fails to reproduce the AES measurements.

摘要

扫描隧道显微镜(STM)、俄歇电子能谱(AES)和低能电子衍射已被用于跟踪不同温度下硅膜在Ag(111)上的生长情况。使用一个简单的生长模型,我们模拟了不同温度下蒸发过程中膜厚度随覆盖率的分布。在据称会形成多层硅烯的温度范围(470 - 500 K)内,发现与Ag表面活性剂介导生长过程中的AES强度变化和STM测量结果吻合良好,而多层硅烯生长模型无法重现AES测量结果。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/4619/5769081/01adc52dcfe8/Beilstein_J_Nanotechnol-09-48-g002.jpg

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