Rodriguez-Fernandez A, Esposito V, Sanchez D F, Finkelstein K D, Juranic P, Staub U, Grolimund D, Reiche S, Pedrini B
Paul Scherrer Institut, Villigen, Switzerland.
Cornell High Energy Synchrotron Source, Ithaca, NY, USA.
Acta Crystallogr A Found Adv. 2018 Mar 1;74(Pt 2):75-87. doi: 10.1107/S2053273318001419. Epub 2018 Feb 23.
Time-delayed, narrow-band echoes generated by forward Bragg diffraction of an X-ray pulse by a perfect thin crystal are exploited for self-seeding at hard X-ray free-electron lasers. Theoretical predictions indicate that the retardation is strictly correlated to a transverse displacement of the echo pulses. This article reports the first experimental observation of the displaced echoes. The displacements are in good agreement with simulations relying on the dynamical diffraction theory. The echo signals are characteristic for a given Bragg reflection, the structure factor and the probed interplane distance. The reported results pave the way to exploiting the signals as an online diagnostic tool for hard X-ray free-electron laser seeding and for dynamical diffraction investigations of strain at the femtosecond timescale.
由完美薄晶体对X射线脉冲进行前向布拉格衍射产生的延时窄带回波被用于硬X射线自由电子激光的自种子注入。理论预测表明,延迟与回波脉冲的横向位移严格相关。本文报道了对位移回波的首次实验观测。这些位移与基于动态衍射理论的模拟结果吻合良好。回波信号对于给定的布拉格反射、结构因子和探测的晶面间距具有特征性。所报道的结果为将这些信号用作硬X射线自由电子激光种子注入的在线诊断工具以及在飞秒时间尺度上进行应变的动态衍射研究铺平了道路。