Rodriguez-Fernandez Angel, Diaz Ana, Iyer Anand H S, Verezhak Mariana, Wakonig Klaus, Colliander Magnus H, Carbone Dina
European X-Ray Free Electron Laser GmbH, Schenefeld DE-22869, Germany.
Paul Scherrer Institute, Forschungsstrasse 111, Villigen PSI, Switzerland CH-5232.
Phys Rev Lett. 2021 Oct 8;127(15):157402. doi: 10.1103/PhysRevLett.127.157402.
Dynamical diffraction effects in thin single crystals produce highly monochromatic parallel x-ray beams with a mutual separation of a few microns and a time delay of a few femtoseconds-the so-called echoes. This ultrafast diffraction effect is used at X-Ray Free Electron Lasers in self-seeding schemes to improve beam monochromaticity. Here, we present a coherent x-ray imaging measurement of echoes from Si crystals and demonstrate that a small surface strain can be used to tune their temporal delay. These results represent a first step toward the ambitious goal of strain tailoring new x-ray optics and, conversely, open up the possibility of using ultrafast dynamical diffraction effects to study strain in materials.
薄单晶中的动态衍射效应可产生高度单色的平行X射线束,其相互间距为几微米,时间延迟为几飞秒——即所谓的回波。这种超快衍射效应在X射线自由电子激光的自种子方案中用于提高光束单色性。在此,我们展示了对硅晶体回波的相干X射线成像测量,并证明小的表面应变可用于调节其时间延迟。这些结果是朝着定制新型X射线光学器件这一宏伟目标迈出的第一步,反之,也开启了利用超快动态衍射效应研究材料应变的可能性。