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2013-2016 年中国西部某石化工业城市颗粒物和气态污染物。

Particulate and gaseous pollutants in a petrochemical industrialized valley city, Western China during 2013-2016.

机构信息

Key Laboratory of Western China's Environmental Systems (Ministry of Education), College of Earth and Environmental Sciences, Lanzhou University, Lanzhou, 730000, China.

State Key Laboratory of Cryospheric Science/Tien Shan Glaciological Station, Northwest Institute of Eco-Environment and Resources, Chinese Academy of Sciences, Lanzhou, 730000, China.

出版信息

Environ Sci Pollut Res Int. 2018 May;25(15):15174-15190. doi: 10.1007/s11356-018-1670-6. Epub 2018 Mar 20.

Abstract

Airborne pollutant characteristics, potential sources, and variation trends of cause are investigated based on the hourly air concentrations of gaseous pollutants and particulate matter from 2013 to 2016 in Lanzhou. The mean concentration of SO, NO, CO, 8-hO, PM, and PM was 25.2 ± 16.0 μg m, 46.5 ± 21.1 μg m, 1.3 ± 0.7 mg m, 77.8 ± 45.5 μg m, 58.7 ± 32.9 μg m, and 131.1 ± 86.2 μg m, respectively. The concentrations of SO, PM, and PM present decreasing trends while NO, CO, and O present increasing trends. PM is the most frequent major pollutants with much higher value than standard limit. However, NO pollution had obvious trends to reach the limit and was more serious in Lanzhou compared with other Chinese cities. Relationship between air pollutants and meteorological parameters suggested that lower primary pollutants were associated with higher wind speed from north and west. Modeled back trajectory demonstrated that the transport of air masses from the Hexi Corridor and Inner Mongolia was responsible for the high concentrations of the air pollutants in wintertime, and high PM level in springtime was related to long-range transport of dust from desert areas of the Sinkiang and the Central Asia. Effects of local pollutant emissions and meteorological condition were preliminary analyzed. Improvement of air quality might be related to the decreasing of pollutant emissions due to strict emissions controls, and the contribution of meteorological condition was not explicit and should be further investigated.

摘要

基于 2013 年至 2016 年兰州小时气态污染物和颗粒物浓度数据,研究了空气污染物特征、潜在来源和变化趋势。SO、NO、CO、8-hO、PM 和 PM 的平均浓度分别为 25.2 ± 16.0 μg m、46.5 ± 21.1 μg m、1.3 ± 0.7 mg m、77.8 ± 45.5 μg m、58.7 ± 32.9 μg m 和 131.1 ± 86.2 μg m。SO、PM 和 PM 的浓度呈下降趋势,而 NO、CO 和 O 的浓度呈上升趋势。PM 是最常见的主要污染物,其浓度值远高于标准限值。然而,NO 污染有明显的达标趋势,且在兰州比其他中国城市更为严重。空气质量污染物与气象参数的关系表明,来自北方和西部的高风速与低浓度的一次污染物有关。后向轨迹模型表明,河西走廊和内蒙古地区的气团输送是造成冬季空气污染物高浓度的原因,而春季高 PM 水平则与来自新疆和中亚沙漠地区的远距离输运有关。初步分析了本地污染物排放和气象条件的影响。空气质量的改善可能与排放控制严格导致的污染物排放减少有关,气象条件的贡献不明显,应进一步研究。

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