Department of Plant Biology, University of Georgia, Athens, GA, United States of America.
Department of Chemistry, University of Georgia, Athens, GA, United States of America.
PLoS One. 2018 Apr 4;13(4):e0194532. doi: 10.1371/journal.pone.0194532. eCollection 2018.
Wood represents the most abundant biomass produced by plants and one of its major components is acetyl xylan. Acetylation in xylan can occur at O-2 or O-3 of a xylosyl residue, at both O-2 and O-3 of a xylosyl residue, and at O-3 of a xylosyl residue substituted at O-2 with glucuronic acid. Acetyltransferases responsible for the regiospecific acetylation of xylan in tree species have not yet been characterized. Here we report the biochemical characterization of twelve Populus trichocarpa DUF231-containing proteins, named PtrXOATs, for their roles in the regiospecific acetylation of xylan. The PtrXOAT genes were found to be differentially expressed in Populus organs and among them, PtrXOAT1, PtrXOAT2, PtrXOAT9 and PtrXOAT10 exhibited the highest level of expression in stems undergoing wood formation. Activity assays of recombinant proteins demonstrated that all twelve PtrXOAT proteins were able to transfer acetyl groups from acetyl CoA onto a xylohexaose acceptor with PtrXOAT1, PtrXOAT2, PtrXOAT3, PtrXOAT11 and PtrXOAT12 having the highest activity. Structural analysis of the PtrXOAT-catalyzed reaction products using 1H NMR spectroscopy revealed that PtrXOAT1, PtrXAOT2 and PtrXOAT3 mediated 2-O- and 3-O-monoacetylation and 2,3-di-O-acetylation of xylosyl residues and PtrXOAT11 and PtrXOAT12 only catalyzed 2-O- and 3-O-monoacetylation of xylosyl residues. Of the twelve PtrXOATs, only PtrXOAT9 and PtrXOAT10 were capable of transferring acetyl groups onto the O-3 position of 2-O-glucuronic acid-substituted xylosyl residues. Furthermore, when expressed in the Arabidopsis eskimo1 mutant, PtrXOAT1, PtrXAOT2 and PtrXOAT3 were able to rescue the defects in xylan acetylation. Together, these results demonstrate that the twelve PtrXOATs are acetyltransferases with different roles in xylan acetylation in P. trichocarpa.
木材代表了植物产生的最丰富的生物质,其主要成分之一是乙酰木聚糖。木聚糖中的乙酰化可以发生在木糖基残基的 O-2 或 O-3 位,在木糖基残基的 O-2 和 O-3 位,以及在被葡萄糖醛酸取代的 O-2 的 O-3 位。负责树木物种中木聚糖区域特异性乙酰化的乙酰基转移酶尚未被表征。在这里,我们报道了十二种含有 Populus trichocarpa DUF231 的蛋白(命名为 PtrXOATs)的生化特征,它们在木聚糖的区域特异性乙酰化中起作用。发现 PtrXOAT 基因在杨树器官中差异表达,其中 PtrXOAT1、PtrXOAT2、PtrXOAT9 和 PtrXOAT10 在正在形成木材的茎中表达水平最高。重组蛋白的活性测定表明,所有十二种 PtrXOAT 蛋白都能够将乙酰基从乙酰辅酶 A 转移到木糖己糖接受体上,其中 PtrXOAT1、PtrXOAT2、PtrXOAT3、PtrXOAT11 和 PtrXOAT12 的活性最高。使用 1H NMR 光谱学对 PtrXOAT 催化反应产物的结构分析表明,PtrXOAT1、PtrXAOT2 和 PtrXOAT3 介导了木糖基残基的 2-O-和 3-O-单乙酰化和 2,3-二-O-乙酰化,而 PtrXOAT11 和 PtrXOAT12 仅催化木糖基残基的 2-O-和 3-O-单乙酰化。在这十二种 PtrXOAT 中,只有 PtrXOAT9 和 PtrXOAT10 能够将乙酰基转移到 2-O-葡萄糖醛酸取代的木糖基残基的 O-3 位。此外,当在拟南芥 eskimo1 突变体中表达时,PtrXOAT1、PtrXAOT2 和 PtrXOAT3 能够挽救木聚糖乙酰化缺陷。总之,这些结果表明,这十二种 PtrXOAT 是乙酰基转移酶,在 P. trichocarpa 中在木聚糖乙酰化中具有不同的作用。