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原子尺度接触中的远程热耗散。

Remote heat dissipation in atom-sized contacts.

作者信息

Tsutsui Makusu, Morikawa Takanori, Yokota Kazumichi, Taniguchi Masateru

机构信息

The Institute of Scientific and Industrial Research, Osaka University, 8-1 Mihogaoka, Ibaraki, Osaka, 567-0047, Japan.

出版信息

Sci Rep. 2018 May 18;8(1):7842. doi: 10.1038/s41598-018-26203-z.

Abstract

Understanding and control of heat dissipation is an important challenge in nanoelectronics wherein field-accelerated hot carriers in current-carrying ballistic systems release a large part of the kinetic energy into external bulk phonon baths. Here we report on a physical mechanism of this remote heat dissipation and its role on the stability of atomic contacts. We used a nano-fabricated thermocouple to directly characterize the self-heating in a mechanically-configurable Au junction. We found more pronounced heat dissipation at the current downstream that signifies the electron-hole asymmetry in Au nanocontacts. Meanwhile, the simultaneously measured single-atom chain lifetime revealed a minor influence of the heat dissipation on the contact stability by virtue of microleads serving as an effective heat spreader to moderate the temperature rise to several Kelvins from the ambient under microwatt input power. The present finding can be used for practical design of atomic and molecular electronic devices for heat dissipation managements.

摘要

在纳米电子学中,理解和控制热耗散是一项重大挑战,在载流弹道系统中,场加速热载流子会将大部分动能释放到外部体声子浴中。在此,我们报告这种远程热耗散的物理机制及其对原子接触稳定性的作用。我们使用纳米制造的热电偶直接表征机械可配置金结中的自热现象。我们发现在电流下游有更明显的热耗散,这表明金纳米接触中存在电子 - 空穴不对称性。同时,同步测量的单原子链寿命显示,由于微引线作为有效的热扩散器,在微瓦输入功率下能将温度从环境温度升高几开尔文,热耗散对接触稳定性的影响较小。本研究结果可用于原子和分子电子器件散热管理的实际设计。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/0b3d/5959854/105b6d9f179e/41598_2018_26203_Fig1_HTML.jpg

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