Department of Physics, Kansas State University, Manhattan, Kansas 66506, USA.
Phys Rev Lett. 2018 Jun 1;120(22):223903. doi: 10.1103/PhysRevLett.120.223903.
We propose a scheme for the reconstruction of plasmonic near fields at isolated nanoparticles from infrared-streaked extreme-ultraviolet photoemission spectra. Based on quantum-mechanically modeled spectra, we demonstrate and analyze the accurate imaging of the IR-streaking-pulse-induced transient plasmonic fields at the surface of gold nanospheres and nanoshells with subfemtosecond temporal and subnanometer spatial resolution.
我们提出了一种从孤立纳米粒子的红外条纹太赫兹光电子能谱中重建等离子体近场的方案。基于量子力学模拟的光谱,我们演示并分析了亚飞秒时间和亚纳米空间分辨率下金纳米球和纳米壳表面的红外条纹脉冲诱导瞬态等离子体场的精确成像。