Burnett Jonathan L, Milbrath Brian D
Pacific Northwest National Laboratory, PO Box 999, Richland, WA, USA.
Pacific Northwest National Laboratory, PO Box 999, Richland, WA, USA.
J Environ Radioact. 2018 Dec;192:160-165. doi: 10.1016/j.jenvrad.2018.06.007. Epub 2018 Jun 28.
There remain technical challenges for an On-site Inspection (OSI) in the high seas environment, which gathers evidence of a violation of the Comprehensive Nuclear-Test-Ban Treaty (CTBT). For terrestrial nuclear explosions, the radionuclide observables are well defined and States Parties have chosen 17 particulate radionuclides that allow discrimination from other nuclear events. However, an underwater nuclear explosion generates induced radionuclides from the neutron activation of seawater, which has the potential to interfere with the measurement of the radionuclide observables using gamma-spectrometry techniques. To understand these effects the inventory of OSI relevant (6.0 × 10 Bq) and activation (1.6 × 10 Bq) radionuclides has been calculated for a 1 kT underwater nuclear explosion. The activation products consist predominantly of Cl and Na, which decay to 5.56% and 0.0007% of their initial activity within 1 and 14 days. Monte Carlo techniques have been used to assess spectral interferences within this timeframe. It is demonstrated that during this period they do not interfere with the measurement of the existing radionuclide observables. Additionally, Na has been identified as useful for inspection purposes.
在公海环境中进行现场视察(OSI)以收集违反《全面禁止核试验条约》(CTBT)的证据仍存在技术挑战。对于陆地核爆炸,放射性核素观测值定义明确,缔约国已选定17种微粒放射性核素,可用于与其他核事件进行区分。然而,水下核爆炸会使海水经中子活化产生感生放射性核素,这有可能干扰利用伽马能谱技术对放射性核素观测值的测量。为了解这些影响,已针对1千吨级水下核爆炸计算了与现场视察相关的(6.0×10贝克勒尔)和活化(1.6×10贝克勒尔)放射性核素的存量。活化产物主要由氯和钠组成,它们在1天和14天内分别衰减至其初始活度的5.56%和0.0007%。已使用蒙特卡罗技术评估该时间段内的光谱干扰。结果表明,在此期间它们不会干扰现有放射性核素观测值的测量。此外,钠已被确定对视察有用。