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不同测量锶(Sr)和锶(Sr)方法的评估:不同方法的测量不确定度作为活度比的函数。

Evaluation of different methods for measuring Sr and Sr: Measurement uncertainty for the different methods as a function of the activity ratio.

作者信息

Rondahl Stina Holmgren, Ramebäck Henrik

机构信息

Swedish Defence Research Agency (FOI), CBRN Defence and Security, Cementvägen 20, 901 82 Umeå, Sweden.

Swedish Defence Research Agency (FOI), CBRN Defence and Security, Cementvägen 20, 901 82 Umeå, Sweden; Chalmers University of Technology, Department of Chemistry and Chemical Engineering, Nuclear Chemistry, 412 96 Göteborg, Sweden.

出版信息

Appl Radiat Isot. 2018 Oct;140:87-95. doi: 10.1016/j.apradiso.2018.06.016. Epub 2018 Jun 20.

Abstract

In case of a radiological emergency situation involving e.g. fission of uranium or plutonium, analysis of radioactive strontium will be of importance. The primary radionuclides of interest are Sr, its progeny Y and Sr. A few days following an event, Sr will be the predominant radioisotope of strontium. Most methods found in the literature are valid and applicable when measuring Sr, but when samples contain both Sr/Sr interference problematics arise. How these interferences are dealt with will have an effect on the uncertainty of the Sr determination. This work aims at evaluating three measurement approaches, all mentioned in the literature, with respect to the measurement uncertainty when determining Sr in an emergency preparedness situation and to propose a suitable measurement strategy.

摘要

在涉及例如铀或钚裂变的放射性紧急情况中,放射性锶的分析将具有重要意义。主要关注的放射性核素是锶-89、其衰变产物钇-89和锶-90。事件发生几天后,锶-90将成为锶的主要放射性同位素。文献中发现的大多数方法在测量锶-90时都是有效的且适用的,但当样品同时含有锶-89/锶-90时,就会出现干扰问题。如何处理这些干扰将影响锶-90测定的不确定度。这项工作旨在评估文献中提到的三种测量方法在应急准备情况下测定锶-90时的测量不确定度,并提出一种合适的测量策略。

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