Laboratory for Aviation and the Environment , Massachusetts Institute of Technology , 77 Massachusetts Avenue , Cambridge , Massachusetts 02139 , United States.
Centre for Environmental Sciences , Hasselt University , Campus Diepenbeek, Agoralaan Gebouw D , 3590 Diepenbeek , Belgium.
Environ Sci Technol. 2018 Nov 6;52(21):12055-12065. doi: 10.1021/acs.est.7b04277. Epub 2018 Oct 17.
This paper quantifies and compares the life cycle GHG emissions and costs of production of diesel and jet fuel derived from municipal solid waste (MSW) in the United States via three thermochemical conversion pathways: conventional gasification and Fischer-Tropsch (FT middle distillate, MD), plasma gasification and Fischer-Tropsch (Plasma FT MD), and conventional gasification, catalytic alcohol synthesis, and alcohol-to-jet upgrading (ATJ MD). We use expanded system boundaries to capture the change in existing MSW use and disposal, and account for parameter uncertainty with Monte Carlo simulations. We estimate median life cycle GHG emissions of 32.9, 62.3, and 52.7 gCOe/MJ for FT, Plasma FT and ATJ MD fuels, respectively, compared to a baseline of 90 gCOe/MJ for conventional MD fuels. Median minimum selling prices are estimated at 0.99, 1.78, and 1.20 $ per liter with the probability of achieving a positive net present value of fuel production at market prices of 14%, 0.1% and 7% for FT, Plasma FT and ATJ MD fuels, respectively. If the societal perspective rather than an investor's perspective is evaluated, then the probability of positive net present value of fuel production increases to 93%, 67%, and 92.5% for the FT, Plasma FT, and ATJ MD fuels, respectively.
本文通过三种热化学转化途径(常规气化和费托法(FT 中间馏分,MD)、等离子气化和费托法(等离子 FT MD)以及常规气化、催化醇合成和醇至喷气升级(ATJ MD)),量化和比较了美国通过城市固体废物(MSW)生产的柴油和喷气燃料的生命周期 GHG 排放和生产成本。我们使用扩展的系统边界来捕捉现有 MSW 使用和处置方式的变化,并通过蒙特卡罗模拟来考虑参数不确定性。我们估计 FT、等离子 FT 和 ATJ MD 燃料的生命周期 GHG 排放中位数分别为 32.9、62.3 和 52.7 gCOe/MJ,而常规 MD 燃料的基线为 90 gCOe/MJ。我们估计,在市场价格为 14%、0.1%和 7%的情况下,FT、等离子 FT 和 ATJ MD 燃料的最低销售价格中值分别为 0.99、1.78 和 1.20 美元/升,FT、等离子 FT 和 ATJ MD 燃料生产燃料的净现值为正的概率分别为 93%、67%和 92.5%。如果从社会角度而不是投资者角度进行评估,那么 FT、等离子 FT 和 ATJ MD 燃料生产燃料的净现值为正的概率分别增加到 93%、67%和 92.5%。