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医用同位素生产、研究堆及其对全球氙背景的贡献。

Medical isotope production, research reactors and their contribution to the global xenon background.

作者信息

Hoffman Ian, Berg Rodney

机构信息

Health Canada, Radiation Protection Bureau, 775 Brookfield Rd, Ottawa, K1A 1C1 Canada.

出版信息

J Radioanal Nucl Chem. 2018;318(1):165-173. doi: 10.1007/s10967-018-6128-2. Epub 2018 Aug 25.

DOI:10.1007/s10967-018-6128-2
PMID:30369686
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC6182739/
Abstract

The Comprehensive Nuclear-Test-Ban Treaty (CTBT) bans the testing of nuclear explosive devices underground, in the atmosphere and underwater. Two main technologies, radionuclide and seismo-acoustic monitoring, are deployed in the International Monitoring System used for the verification of the CTBT. Medical isotope production from fission-based processes is the dominant contributor to a worldwide background of radioxenon. This background can make the discrimination of nuclear tests from legitimate nuclear activities very challenging. Even if emissions from medical isotope producers experienced a large reduction, there remain other important sources of radioxenon that contribute to the global background such as research reactors and nuclear power plants. Until recently, the largest producer of medical isotopes was located in Canada, at the Canadian Nuclear Laboratories (CNL) facility. The characterization of CNL emissions and its research reactor can provide valuable information for effective verification of the CTBT.

摘要

《全面禁止核试验条约》(CTBT)禁止在地下、大气层和水下进行核爆炸装置试验。用于核查《全面禁止核试验条约》的国际监测系统采用了两种主要技术,即放射性核素监测和地震声学监测。基于裂变过程的医用同位素生产是全球放射性氙背景的主要来源。这种背景使得区分核试验与合法核活动极具挑战性。即使医用同位素生产者的排放大幅减少,仍存在其他重要的放射性氙来源,如研究堆和核电站,它们也对全球背景有贡献。直到最近,医用同位素的最大生产国是加拿大,生产设施位于加拿大核实验室(CNL)。加拿大核实验室的排放特征及其研究堆可为有效核查《全面禁止核试验条约》提供有价值的信息。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/85f0/6182739/0a092f41b97f/10967_2018_6128_Fig8_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/85f0/6182739/f7b9638139ab/10967_2018_6128_Fig1_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/85f0/6182739/15c171ccadb9/10967_2018_6128_Fig2_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/85f0/6182739/8bbe6e6c61b6/10967_2018_6128_Fig3_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/85f0/6182739/d9db7d225702/10967_2018_6128_Fig4_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/85f0/6182739/d964d0d74f7c/10967_2018_6128_Fig5_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/85f0/6182739/f24d8256884a/10967_2018_6128_Fig6_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/85f0/6182739/a4b467e3024d/10967_2018_6128_Fig7_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/85f0/6182739/0a092f41b97f/10967_2018_6128_Fig8_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/85f0/6182739/f7b9638139ab/10967_2018_6128_Fig1_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/85f0/6182739/15c171ccadb9/10967_2018_6128_Fig2_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/85f0/6182739/8bbe6e6c61b6/10967_2018_6128_Fig3_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/85f0/6182739/d9db7d225702/10967_2018_6128_Fig4_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/85f0/6182739/d964d0d74f7c/10967_2018_6128_Fig5_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/85f0/6182739/f24d8256884a/10967_2018_6128_Fig6_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/85f0/6182739/a4b467e3024d/10967_2018_6128_Fig7_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/85f0/6182739/0a092f41b97f/10967_2018_6128_Fig8_HTML.jpg

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本文引用的文献

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J Environ Radioact. 2014 Apr;130:33-43. doi: 10.1016/j.jenvrad.2013.12.006. Epub 2014 Jan 11.
2
Radioxenon detections in the CTBT international monitoring system likely related to the announced nuclear test in North Korea on February 12, 2013.国际监测系统中的放射性氙检测可能与 2013 年 2 月 12 日朝鲜宣布的核试验有关。
J Environ Radioact. 2014 Feb;128:47-63. doi: 10.1016/j.jenvrad.2013.10.027. Epub 2013 Nov 30.
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Maximum reasonable radioxenon releases from medical isotope production facilities and their effect on monitoring nuclear explosions.
最大合理放射性氙释放量从医疗同位素生产设施及其对监测核爆炸的影响。
J Environ Radioact. 2013 Jan;115:192-200. doi: 10.1016/j.jenvrad.2012.07.018. Epub 2012 Sep 20.
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Isotopic noble gas signatures released from medical isotope production facilities--simulations and measurements.医学同位素生产设施释放的同位素惰性气体特征——模拟与测量
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Atmospheric xenon radioactive isotope monitoring.大气氙放射性同位素监测。
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