Molecular Biophysics Unit, Indian Institute of Science, Bangalore, 560012, India.
INSERM, U 1134, DSIMB, F-75739, Paris, France.
Protein Sci. 2019 Mar;28(3):543-560. doi: 10.1002/pro.3556. Epub 2018 Dec 30.
Many protein kinases are characterized by at least two structural forms corresponding to the highest level of activity (active) and low or no activity, (inactive). Further, protein dynamics is an important consideration in understanding the molecular and mechanistic basis of enzyme function. In this work, we use protein kinase A (PKA) as the model system and perform microsecond range molecular dynamics (MD) simulations on six variants which differ from one another in terms of active and inactive form, with or without bound ligands, C-terminal tail and phosphorylation at the activation loop. We find that the root mean square fluctuations in the MD simulations are generally higher for the inactive forms than the active forms. This difference is statistically significant. The higher dynamics of inactive states has significant contributions from ATP binding loop, catalytic loop, and αG helix. Simulations with and without C-terminal tail show this differential dynamics as well, with lower dynamics both in the active and inactive forms if C-terminal tail is present. Similarly, the dynamics associated with the inactive form is higher irrespective of the phosphorylation status of Thr 197. A relatively stable stature of active kinases may be better suited for binding of substrates and detachment of the product. Also, phosphoryl group transfer from ATP to the phosphosite on the substrate requires precise transient coordination of chemical entities from three different molecules, which may be facilitated by the higher stability of the active state.
许多蛋白激酶的结构至少有两种形式,分别对应于最高活性(活性)和低活性或无活性(非活性)。此外,蛋白质动力学是理解酶功能的分子和机制基础的重要考虑因素。在这项工作中,我们使用蛋白激酶 A(PKA)作为模型系统,并对六种变体进行了微秒范围内的分子动力学(MD)模拟,这些变体在活性和非活性形式、有无结合配体、C 末端尾部和激活环磷酸化方面彼此不同。我们发现,MD 模拟中的均方根波动通常对于非活性形式高于活性形式。这种差异具有统计学意义。非活性状态的高动力学主要来自于 ATP 结合环、催化环和αG 螺旋。有和没有 C 末端尾部的模拟也显示了这种差异动力学,并且如果存在 C 末端尾部,则活性和非活性形式的动力学都较低。同样,与 Thr197 的磷酸化状态无关,非活性形式的动力学更高。活性激酶的相对稳定状态可能更适合于与底物结合和产物释放。此外,从 ATP 向底物上的磷酸化位点转移磷酸基团需要来自三个不同分子的化学实体的精确瞬时协调,这可能通过活性状态的更高稳定性来促进。