Beye M, Engel R Y, Schunck J O, Dziarzhytski S, Brenner G, Miedema P S
Deutsches Elektronen Synchrotron DESY, Notkestr. 85, 22607 Hamburg, Germany. Physics Department, Universität Hamburg, Luruper Chaussee 149, 22761 Hamburg, Germany.
J Phys Condens Matter. 2019 Jan 9;31(1):014003. doi: 10.1088/1361-648X/aaedf3.
With the intense and coherent x-ray pulses available from free-electron lasers, the possibility to transfer non-linear spectroscopic methods from the laser lab to the x-ray world arises. Advantages especially regarding selectivity and thus information content as well as an improvement of signal levels are expected. The use of coherences is especially fruitful and the example of coherent x-ray/optical sum-frequency generation is discussed. However, many non-linear x-ray methods still await discovery, partially due to the necessity for extremely adaptable and versatile instrumentation that can be brought to free-electron lasers for the analysis of the spectral content emitted from the sample into a continuous range of emission angles. Such an instrument (called MUSIX) is being developed and employed at FLASH, the free-electron laser in Hamburg and is described in this contribution together with first results.
利用自由电子激光产生的高强度且相干的X射线脉冲,出现了将非线性光谱方法从激光实验室转移到X射线领域的可能性。预计尤其在选择性以及信息含量方面具有优势,同时信号水平也会得到提高。相干性的利用特别富有成效,并讨论了相干X射线/光学和频产生的例子。然而,许多非线性X射线方法仍有待发现,部分原因是需要极其灵活通用的仪器,该仪器可用于自由电子激光,以便将样品发射的光谱内容分析到连续的发射角范围内。这样一种仪器(称为MUSIX)正在汉堡的自由电子激光FLASH上进行开发和使用,本论文将对其进行描述并给出初步结果。