Minnesota Department of Health, Saint Paul, MN, USA.
J Expo Sci Environ Epidemiol. 2019 Mar;29(2):218-226. doi: 10.1038/s41370-018-0101-6. Epub 2018 Dec 5.
The Minnesota Department of Health measured levels of perfluoroalkyl acids (PFAAs) in house dust at homes in communities impacted by PFAA-contaminated soil and drinking water to determine whether PFAAs in soil outside the home are associated with concentrations in dust. House dust samples from both interior living spaces and entryways to the yard were collected and analyzed separately based on the presumption that PFAAs in entryway dust may better reflect "track-in" of PFAAs into the home from contaminated soil or lawns irrigated with contaminated water. PFAA detections and concentrations in living rooms were significantly higher compared to entryways; and concentrations in both sampling locations were higher than corresponding soil concentrations, suggesting that interior sources were the main contributors to PFAAs in house dust. PFAA dust concentrations in entryways were significantly associated with living room dust levels for all analytes except PFBA. Relationships between entryway dust and soil were only seen for one PFAA (PFOA). However, median concentrations of PFOA in entryway and living room dust were 35 and 70 times higher (respectively) than in soil, which highlights the lack of importance of PFAA soil track-in as a contributor to dust concentration in this setting. Due to the small sample size, larger scale studies are needed to further assess the potential for migration of PFAA contaminated soil to indoor dust.
明尼苏达州公共卫生部在受全氟烷基酸(PFAAs)污染土壤和饮用水影响的社区的家庭中测量了房屋灰尘中的 PFAAs 水平,以确定家庭以外的土壤中的 PFAAs 是否与灰尘中的浓度有关。根据假设,从污染土壤或受污染水灌溉的草坪“带入”家中的 PFAAs 可能更好地反映在入口灰尘中的“带入”,分别收集和分析了来自内部居住空间和通往院子入口的房屋灰尘样本。与入口处相比,客厅中的 PFAA 检测和浓度明显更高;并且两个采样地点的浓度均高于相应的土壤浓度,这表明室内来源是房屋灰尘中 PFAAs 的主要来源。除了 PFBA 之外,所有分析物的入口处灰尘与客厅灰尘水平均呈显著相关。仅在一种 PFAA(全氟辛酸)中观察到入口处灰尘与土壤之间的关系。然而,入口处和客厅灰尘中 PFOA 的中位数浓度分别比土壤高 35 倍和 70 倍(分别),这突出表明在这种情况下,PFAA 土壤“带入”作为灰尘浓度的贡献者的重要性不大。由于样本量较小,需要更大规模的研究来进一步评估 PFAA 污染土壤向室内灰尘迁移的潜力。