Horvath Thomas D, Chan Wai Kin, Pontikos Michael A, Martin Leona A, Du Di, Tan Lin, Konopleva Marina, Weinstein John N, Lorenzi Philip L
Department of Bioinformatics and Computational Biology and The Proteomics and Metabolomics Core Facility, The University of Texas MD Anderson Cancer Center, Houston, TX 77030, USA.
Department of Leukemia, The University of Texas MD Anderson Cancer Center, Houston, TX 77030, USA.
Metabolites. 2019 Jan 9;9(1):10. doi: 10.3390/metabo9010010.
l-asparaginase (ASNase) is a metabolism-targeted anti-neoplastic agent used to treat acute lymphoblastic leukemia (ALL). ASNase's anticancer activity results from the enzymatic depletion of asparagine (Asn) and glutamine (Gln), which are converted to aspartic acid (Asp) and glutamic acid (Glu), respectively, in the blood. Unfortunately, accurate assessment of the in vivo pharmacodynamics (PD) of ASNase is challenging because of the following reasons: (i) ASNase is resilient to deactivation; (ii) ASNase catalytic efficiency is very high; and (iii) the PD markers Asn and Gln are depleted ex vivo in blood samples containing ASNase. To address those issues and facilitate longitudinal studies in individual mice for ASNase PD studies, we present here a new LC-MS/MS bioanalytical method that incorporates rapid quenching of ASNase for measurement of Asn, Asp, Gln, and Glu in just 10 µL of whole blood, with limits of detection (s:n ≥ 10:1) estimated to be 2.3, 3.5, 0.8, and 0.5 µM, respectively. We tested the suitability of the method in a 5-day, longitudinal PD study in mice and found the method to be simple to perform with sufficient accuracy and precision for whole blood measurements. Overall, the method increases the density of data that can be acquired from a single animal and will facilitate optimization of novel ASNase treatment regimens and/or the development of new ASNase variants with desired kinetic properties.
L-天冬酰胺酶(ASNase)是一种靶向代谢的抗肿瘤药物,用于治疗急性淋巴细胞白血病(ALL)。ASNase的抗癌活性源于天冬酰胺(Asn)和谷氨酰胺(Gln)的酶促消耗,它们在血液中分别转化为天冬氨酸(Asp)和谷氨酸(Glu)。不幸的是,由于以下原因,准确评估ASNase的体内药效学(PD)具有挑战性:(i)ASNase对失活具有抗性;(ii)ASNase的催化效率非常高;(iii)PD标志物Asn和Gln在含有ASNase的血液样本中离体时会被消耗。为了解决这些问题并促进对单个小鼠进行ASNase PD研究的纵向研究,我们在此介绍一种新的LC-MS/MS生物分析方法,该方法结合了对ASNase的快速淬灭,可在仅10 μL全血中测量Asn、Asp、Gln和Glu,估计检测限(s:n≥10:1)分别为2.3、3.5、0.8和0.5 μM。我们在一项为期5天的小鼠纵向PD研究中测试了该方法的适用性,发现该方法操作简单,对全血测量具有足够的准确性和精密度。总体而言,该方法增加了可从单个动物获得的数据密度,并将有助于优化新型ASNase治疗方案和/或开发具有所需动力学特性的新型ASNase变体。