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自推进系统中的活性去局域化和冻结。

Activity induced delocalization and freezing in self-propelled systems.

机构信息

Gran Sasso Science Institute (GSSI), Via. F. Crispi 7, 67100, L'Aquila, Italy.

Scuola di Scienze e Tecnologie, Università di Camerino - via Madonna delle Carceri, 62032, Camerino, Italy.

出版信息

Sci Rep. 2019 Feb 4;9(1):1386. doi: 10.1038/s41598-018-36824-z.

DOI:10.1038/s41598-018-36824-z
PMID:30718579
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC6361910/
Abstract

We study a system of interacting active particles, propelled by colored noises, characterized by an activity time τ, and confined by a single-well anharmonic potential. We assume pair-wise repulsive forces among particles, modelling the steric interactions among microswimmers. This system has been experimentally studied in the case of a dilute suspension of Janus particles confined through acoustic traps. We observe that already in the dilute regime - when inter-particle interactions are negligible - increasing the persistent time, τ, pushes the particles away from the potential minimum, until a saturation distance is reached. We compute the phase diagram (activity versus interaction length), showing that the interaction does not suppress this delocalization phenomenon but induces a liquid- or solid-like structure in the densest regions. Interestingly a reentrant behavior is observed: a first increase of τ from small values acts as an effective warming, favouring fluidization; at higher values, when the delocalization occurs, a further increase of τ induces freezing inside the densest regions. An approximate analytical scheme gives fair predictions for the density profiles in the weakly interacting case. The analysis of non-equilibrium heat fluxes reveals that in the region of largest particle concentration equilibrium is restored in several aspects.

摘要

我们研究了一个由有色噪声驱动的相互作用的活性粒子系统,其特征是活动时间 τ,并受到单阱非谐势的限制。我们假设粒子之间存在相互排斥的力,从而模拟微泳者之间的空间相互作用。在含有声阱限制的 Janus 粒子稀悬浮液的情况下,已经对该系统进行了实验研究。我们观察到,即使在稀相中 - 当粒子间相互作用可以忽略不计 - 增加持续时间 τ 也会将粒子推离势阱最小值,直到达到饱和距离。我们计算了相图(活性与相互作用长度),结果表明相互作用不会抑制这种离域现象,而是在最密集的区域中诱导出液体或固体状结构。有趣的是,观察到了一种再进入行为:从较小值开始增加 τ 会起到有效的升温作用,有利于流化;在更高的值下,当发生离域时,进一步增加 τ 会在最密集的区域中引起冻结。近似分析方案可以对弱相互作用情况下的密度分布进行合理预测。对非平衡热通量的分析表明,在最大粒子浓度区域,从多个方面恢复了平衡。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a28f/6361910/3da449989a1b/41598_2018_36824_Fig3_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a28f/6361910/ce62a7102992/41598_2018_36824_Fig1_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a28f/6361910/1434ede01506/41598_2018_36824_Fig2_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a28f/6361910/3da449989a1b/41598_2018_36824_Fig3_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a28f/6361910/ce62a7102992/41598_2018_36824_Fig1_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a28f/6361910/1434ede01506/41598_2018_36824_Fig2_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a28f/6361910/3da449989a1b/41598_2018_36824_Fig3_HTML.jpg

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本文引用的文献

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Comment on "Entropy Production and Fluctuation Theorems for Active Matter".对《活性物质的熵产生与涨落定理》的评论
Phys Rev Lett. 2018 Sep 28;121(13):139801. doi: 10.1103/PhysRevLett.121.139801.
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Full Phase Diagram of Active Brownian Disks: From Melting to Motility-Induced Phase Separation.活性布朗磁盘的全相图:从熔融到运动诱导的相分离。
Phys Rev Lett. 2018 Aug 31;121(9):098003. doi: 10.1103/PhysRevLett.121.098003.
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A random first-order transition theory for an active glass.活性玻璃的随机一阶转变理论。
Proc Natl Acad Sci U S A. 2018 Jul 24;115(30):7688-7693. doi: 10.1073/pnas.1721324115. Epub 2018 Jul 9.
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Memory-less response and violation of the fluctuation-dissipation theorem in colloids suspended in an active bath.无记忆响应和违反涨落耗散定理的胶体悬浮在活跃的浴中。
Sci Rep. 2017 Dec 14;7(1):17588. doi: 10.1038/s41598-017-17900-2.
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Heat, temperature and Clausius inequality in a model for active Brownian particles.活性布朗粒子模型中的热、温度与克劳修斯不等式
Sci Rep. 2017 Apr 21;7:46496. doi: 10.1038/srep46496.
6
Escape rate of active particles in the effective equilibrium approach.有效平衡方法中活性粒子的逃逸率。
Phys Rev E. 2017 Jan;95(1-1):012115. doi: 10.1103/PhysRevE.95.012115. Epub 2017 Jan 10.
7
The nonequilibrium glassy dynamics of self-propelled particles.自推进粒子的非平衡玻璃动力学。
Soft Matter. 2016 Sep 14;12(34):7136-49. doi: 10.1039/c6sm01322h. Epub 2016 Aug 8.
8
How Far from Equilibrium Is Active Matter?活性物质离平衡态有多远?
Phys Rev Lett. 2016 Jul 15;117(3):038103. doi: 10.1103/PhysRevLett.117.038103. Epub 2016 Jul 13.
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Control of active liquid crystals with a magnetic field.利用磁场控制活性液晶
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Velocity distribution in active particles systems.活性粒子系统中的速度分布。
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