Department of Materials Science and Engineering, Yonsei University, Seoul, 03722, Korea.
Center for Multi-Dimensional Materials, Yonsei University, Seoul, 03722, Korea.
Nat Commun. 2019 Feb 8;10(1):653. doi: 10.1038/s41467-019-08552-z.
The ideal combination of high optical transparency and high electrical conductivity, especially at very low frequencies of less than the gigahertz (GHz) order, such as the radiofrequencies at which electronic devices operate (tens of kHz to hundreds of GHz), is fundamental incompatibility, which creates a barrier to the realization of enhanced user interfaces and 'device-to-device integration.' Herein, we present a design strategy for preparing a megahertz (MHz)-transparent conductor, based on a plasma frequency controlled by the electrical conductivity, with the ultimate goal of device-to-device integration through electromagnetic wave transmittance. This approach is verified experimentally using a conducting polymer, poly(3,4-ethylenedioxythiophene)-poly(styrenesulfonate) (PEDOT:PSS), the microstructure of which is manipulated by employing a solution process. The use of a transparent conducting polymer as an electrode enables the fabrication of a fully functional touch-controlled display device and magnetic resonance imaging (MRI)-compatible biomedical monitoring device, which would open up a new paradigm for transparent conductors.
高光学透明度和高导电性的理想结合,特别是在低于千兆赫(GHz)频率的情况下,例如电子设备工作的射频频率(几十千赫兹到几百 GHz),是一种基本的不兼容性,这给增强型用户界面和“设备到设备集成”的实现带来了障碍。在此,我们提出了一种基于等离子体频率受电导率控制的兆赫兹(MHz)透明导体的设计策略,其最终目标是通过电磁波透射实现设备到设备的集成。我们通过使用导电聚合物聚(3,4-亚乙基二氧噻吩)-聚(苯乙烯磺酸盐)(PEDOT:PSS)实验验证了这种方法,该聚合物的微观结构通过溶液处理进行了操纵。使用透明导电聚合物作为电极可以制造出完全功能的触摸控制显示设备和磁共振成像(MRI)兼容的生物医学监测设备,这将为透明导体开辟一个新的范例。