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冬季干旱对中国西南地区空气污染的影响。

Impact of winter droughts on air pollution over Southwest China.

机构信息

Key Laboratory of Arid Climate Change and Reducing Disaster in Gansu Province, College of Atmospheric Sciences, Lanzhou University, Lanzhou 730000, China.

Key Laboratory of Arid Climate Change and Reducing Disaster in Gansu Province, College of Atmospheric Sciences, Lanzhou University, Lanzhou 730000, China; Plateau Atmosphere and Environment Key Laboratory of Sichuan Province, College of Atmospheric Sciences, Chengdu University of Information Technology, Chengdu 610225, China.

出版信息

Sci Total Environ. 2019 May 10;664:724-736. doi: 10.1016/j.scitotenv.2019.01.335. Epub 2019 Jan 28.

Abstract

The meteorological causes of winter droughts over Southwest China (SWC) have been widely investigated in recent years; however, little information is available on the impact of these droughts on air pollution. This study (1) characterized and quantified the impact of winter droughts on air pollution over SWC and (2) investigated the atmospheric teleconnections associated with the winter droughts in this region using air pollution monitoring data, routinely observed meteorological data, and National Centers for Environmental Prediction/National Center for Atmospheric Research and ERA-Interim reanalysis data. The main results are as follows: (1) A surface high pressure system together with a weak descent in the middle troposphere was the main cause of the SWC drought in December 2017. (2) It has been found that precipitation, the number of precipitation days and the atmospheric boundary layer height all decreased during the droughts, resulting in unfavorable conditions for the dispersion of air pollutants. (3) The concentrations of PM and PM were much higher during dry periods than those during non-dry periods over SWC, especially in the Sichuan Basin of the SWC. (4) WRF-Chem simulations reproduced the observed changes in air pollutant concentrations between dry and non-dry conditions. (5) Atmospheric teleconnections associated with the winter droughts in SWC were negative phases of the conventional Eurasian teleconnection, Eastern Atlantic/Western Russia pattern, Arctic Oscillation and North Atlantic Oscillation, and a La Niña event. Overall, this study provides scientific support for the long-term potential and accurate short-term predictions of air pollution in SWC.

摘要

近年来,人们广泛研究了中国西南地区(SWC)冬季干旱的气象成因,但关于这些干旱对空气污染影响的信息却很少。本研究(1)描述并量化了冬季干旱对 SWC 地区空气污染的影响,(2)利用空气污染监测数据、常规观测气象数据以及美国国家环境预报中心/美国国家大气研究中心和 ERA-Interim 再分析数据,调查了与该地区冬季干旱相关的大气遥相关关系。主要结果如下:(1)表面高压系统和中层弱下沉气流是导致 2017 年 12 月 SWC 干旱的主要原因。(2)研究发现,降水、降水日数和大气边界层高度在干旱期间均下降,导致空气污染物扩散的不利条件。(3)在 SWC 地区,特别是在四川盆地,干旱期间的 PM 和 PM 浓度明显高于非干旱期间。(4)WRF-Chem 模拟再现了观测到的空气污染物浓度在干旱和非干旱条件下的变化。(5)与 SWC 冬季干旱相关的大气遥相关关系为常规欧亚遥相关、东大西洋/俄罗斯西部型、北极涛动和北大西洋涛动的负位相,以及拉尼娜事件。总体而言,本研究为 SWC 地区空气污染的长期潜在和准确短期预测提供了科学支持。

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