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机器学习引导发现新型热电材料。

Machine-learning guided discovery of a new thermoelectric material.

作者信息

Iwasaki Yuma, Takeuchi Ichiro, Stanev Valentin, Kusne Aaron Gilad, Ishida Masahiko, Kirihara Akihiro, Ihara Kazuki, Sawada Ryohto, Terashima Koichi, Someya Hiroko, Uchida Ken-Ichi, Saitoh Eiji, Yorozu Shinichi

机构信息

Central Research Laboratories, NEC Corporation, Tsukuba, 305-8501, Japan.

PRESTO, JST, Saitama, 322-0012, Japan.

出版信息

Sci Rep. 2019 Feb 26;9(1):2751. doi: 10.1038/s41598-019-39278-z.

DOI:10.1038/s41598-019-39278-z
PMID:30808974
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC6391459/
Abstract

Thermoelectric technologies are becoming indispensable in the quest for a sustainable future. Recently, an emerging phenomenon, the spin-driven thermoelectric effect (STE), has garnered much attention as a promising path towards low cost and versatile thermoelectric technology with easily scalable manufacturing. However, progress in development of STE devices is hindered by the lack of understanding of the fundamental physics and materials properties responsible for the effect. In such nascent scientific field, data-driven approaches relying on statistics and machine learning, instead of more traditional modeling methods, can exhibit their full potential. Here, we use machine learning modeling to establish the key physical parameters controlling STE. Guided by the models, we have carried out actual material synthesis which led to the identification of a novel STE material with a thermopower an order of magnitude larger than that of the current generation of STE devices.

摘要

热电技术在追求可持续未来的过程中变得不可或缺。最近,一种新兴现象——自旋驱动热电效应(STE),作为通往低成本、通用且易于扩展制造的热电技术的一条有前途的途径,备受关注。然而,由于对导致该效应的基本物理和材料特性缺乏了解,STE 器件的开发进展受到阻碍。在这样一个新兴的科学领域,依赖统计和机器学习的数据驱动方法,而非更传统的建模方法,能够充分发挥其潜力。在此,我们使用机器学习建模来确定控制 STE 的关键物理参数。在这些模型的指导下,我们进行了实际的材料合成,从而鉴定出一种新型的 STE 材料,其热功率比当前一代 STE 器件大一个数量级。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/4d6b/6391459/b2774e56ffdf/41598_2019_39278_Fig3_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/4d6b/6391459/182ee4ddfef6/41598_2019_39278_Fig1_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/4d6b/6391459/67a26111051c/41598_2019_39278_Fig2_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/4d6b/6391459/b2774e56ffdf/41598_2019_39278_Fig3_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/4d6b/6391459/182ee4ddfef6/41598_2019_39278_Fig1_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/4d6b/6391459/67a26111051c/41598_2019_39278_Fig2_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/4d6b/6391459/b2774e56ffdf/41598_2019_39278_Fig3_HTML.jpg

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1
Machine learning for molecular and materials science.机器学习在分子和材料科学中的应用。
Nature. 2018 Jul;559(7715):547-555. doi: 10.1038/s41586-018-0337-2. Epub 2018 Jul 25.
2
Learning from data to design functional materials without inversion symmetry.从数据中学习设计没有反转对称性的功能材料。
Nat Commun. 2017 Feb 17;8:14282. doi: 10.1038/ncomms14282.
3
Flexible heat-flow sensing sheets based on the longitudinal spin Seebeck effect using one-dimensional spin-current conducting films.基于纵向自旋塞贝克效应、采用一维自旋电流传导薄膜的柔性热流传感片。
连接纳米制造与人工智能——全面综述
Materials (Basel). 2024 Apr 2;17(7):1621. doi: 10.3390/ma17071621.
4
Neural Network for Principle of Least Action.神经网络最小作用量原理。
J Chem Inf Model. 2022 Jul 25;62(14):3346-3351. doi: 10.1021/acs.jcim.2c00515. Epub 2022 Jul 5.
5
Universal machine learning framework for defect predictions in zinc blende semiconductors.用于闪锌矿半导体缺陷预测的通用机器学习框架。
Patterns (N Y). 2022 Feb 14;3(3):100450. doi: 10.1016/j.patter.2022.100450. eCollection 2022 Mar 11.
6
Optimizing machine learning models for granular NdFeB magnets by very fast simulated annealing.通过极快速模拟退火优化用于颗粒钕铁硼磁体的机器学习模型。
Sci Rep. 2021 Feb 15;11(1):3792. doi: 10.1038/s41598-021-83315-9.
7
Model-Free Cluster Analysis of Physical Property Data using Information Maximizing Self-Argument Training.使用信息最大化自论证训练对物理性质数据进行无模型聚类分析。
Sci Rep. 2020 May 13;10(1):7903. doi: 10.1038/s41598-020-64281-0.
8
Predicting material properties by integrating high-throughput experiments, high-throughput ab-initio calculations, and machine learning.通过整合高通量实验、高通量从头算计算和机器学习来预测材料特性。
Sci Technol Adv Mater. 2019 Dec 20;21(1):25-28. doi: 10.1080/14686996.2019.1707111. eCollection 2020.
Sci Rep. 2016 Mar 15;6:23114. doi: 10.1038/srep23114.
4
On-the-fly machine-learning for high-throughput experiments: search for rare-earth-free permanent magnets.用于高通量实验的即时机器学习:寻找无稀土永磁体。
Sci Rep. 2014 Sep 15;4:6367. doi: 10.1038/srep06367.
5
Longitudinal spin Seebeck effect: from fundamentals to applications.纵向自旋塞贝克效应:从基础到应用
J Phys Condens Matter. 2014 Aug 27;26(34):343202. doi: 10.1088/0953-8984/26/34/343202. Epub 2014 Aug 8.
6
Spectral non-uniform temperature and non-local heat transfer in the spin Seebeck effect.自旋塞贝克效应中的谱非均匀温度和非局域热传递。
Nat Commun. 2013;4:1945. doi: 10.1038/ncomms2945.
7
Spin-current-driven thermoelectric coating.自旋电流驱动的热电器件涂层。
Nat Mater. 2012 Jun 17;11(8):686-9. doi: 10.1038/nmat3360.
8
Spin caloritronics.自旋热电子学。
Nat Mater. 2012 Apr 23;11(5):391-9. doi: 10.1038/nmat3301.
9
Intrinsic spin-dependent thermal transport.固有自旋相关热输运。
Phys Rev Lett. 2011 Nov 18;107(21):216604. doi: 10.1103/PhysRevLett.107.216604. Epub 2011 Nov 17.
10
Spin Seebeck insulator.自旋 Seebeck 绝缘体。
Nat Mater. 2010 Nov;9(11):894-7. doi: 10.1038/nmat2856. Epub 2010 Sep 26.