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基于地统计学的 2013-2017 年中国东部地区省级 PM 污染的时空变化及其因素。

Spatio-temporal variations and factors of a provincial PM pollution in eastern China during 2013-2017 by geostatistics.

机构信息

International Center for Ecology, Meteorology, and Environment, Collaborative Innovation Center of Atmospheric Environment and Equipment Technology (AEET), School of Applied Meteorology, Nanjing University of Information Science & Technology, Nanjing, 210044, China.

出版信息

Sci Rep. 2019 Mar 5;9(1):3613. doi: 10.1038/s41598-019-40426-8.

Abstract

Fine particulate matter (PM) is a typical air pollutant and has adverse health effects across the world, especially in the rapidly developing China due to significant air pollution. The PM pollution varies with time and space, and is dominated by the locations owing to the differences in geographical conditions including topography and meteorology, the land use and the characteristics of urbanization and industrialization, all of which control the pollution formation by influencing the various sources and transport of PM. To characterize these parameters and mechanisms, the 5-year PM pollution patterns of Jiangsu province in eastern China with high-resolution was investigated. The Kriging interpolation method of geostatistical analysis (GIS) and the HYbrid Single-Particle Lagrangian Integrated Trajectory (HYSPLIT) model were conducted to study the spatial and temporal distribution of air pollution at 110 sites from national air quality monitoring network covering 13 cities. The PM pollution of the studied region was obvious, although the annual average concentration decreased from previous 72 to recent 50 μg m. Evident temporal variations showed high PM level in winter and low in summer. Spatially, PM level was higher in northern (inland, heavy industry) than that in eastern (costal, plain) regions. Industrial sources contributed highest to the air pollution. Backward trajectory clustering and potential source contribution factor (PSCF) analysis indicated that the typical monsoon climate played an important role in the aerosol transport. In summer, the air mass in Jiangsu was mainly affected by the updraft from near region, which accounted for about 60% of the total number of trajectories, while in winter, the long-distance transport from the northwest had a significant impact on air pollution.

摘要

细颗粒物(PM)是一种典型的空气污染物,对全球健康都有不良影响,尤其是在中国这样空气污染严重、发展迅速的国家。PM 污染随时间和空间变化而变化,由于地理位置的差异,包括地形和气象条件、土地利用以及城市化和工业化的特点,这些因素控制着 PM 的各种来源和传输,从而导致污染形成。为了描述这些参数和机制,对中国东部江苏省进行了为期 5 年的高分辨率 PM 污染模式研究。采用地统计分析(GIS)的克里金插值法和 HYbrid Single-Particle Lagrangian Integrated Trajectory(HYSPLIT)模型,对全国空气质量监测网络覆盖的 13 个城市的 110 个站点的空气污染时空分布进行了研究。研究区域的 PM 污染明显,尽管年平均浓度从之前的 72μg/m3下降到最近的 50μg/m3。明显的时间变化表明冬季 PM 水平较高,夏季较低。空间上,北部(内陆、重工业)地区的 PM 水平高于东部(沿海、平原)地区。工业源对空气污染的贡献最大。后向轨迹聚类和潜在源贡献因子(PSCF)分析表明,典型的季风气候对气溶胶传输起着重要作用。在夏季,江苏的气团主要受近区上升气流的影响,约占轨迹总数的 60%,而在冬季,来自西北的远距离传输对空气污染有显著影响。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/f519/6401087/d24df13f0ca1/41598_2019_40426_Fig1_HTML.jpg

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