Marini Andrea, Ciattoni Alessandro, Conti Claudio
Department of Physical and Chemical Sciences, University of L'Aquila, Via Vetoio, 67100 L'Aquila, Italy.
Faraday Discuss. 2019 May 23;214(0):235-243. doi: 10.1039/c8fd00153g.
We investigate the ultrafast nonlinear response of silver upon excitation by infrared electromagnetic radiation pulses with a duration of a few femtoseconds. By adopting the Landau weak coupling approach to account for electron-electron and electron-phonon collisions, we solve the Boltzmann equation through the method of moments obtaining a novel set of hydrodynamical equations describing the ultrafast nonlinear dynamics of electrons in silver. While the novel hydrodynamical model that was obtained reduces to the Drude model for small intensities of the driving field, it predicts that absorption saturates for large but experimentally attainable peak intensities of the order of GW cm-2. Our results are important for absorption mitigation in plasmonic devices, with potential impact for low-loss plasmonic waveguides and interconnects.
我们研究了银在持续时间为几飞秒的红外电磁辐射脉冲激发下的超快非线性响应。通过采用朗道弱耦合方法来考虑电子 - 电子和电子 - 声子碰撞,我们通过矩量法求解玻尔兹曼方程,得到了一组描述银中电子超快非线性动力学的新型流体动力学方程。虽然所得到的新型流体动力学模型在驱动场强度较小时简化为德鲁德模型,但它预测对于高达GW/cm²量级的大的但在实验上可达到的峰值强度,吸收会饱和。我们的结果对于等离子体器件中的吸收缓解很重要,对低损耗等离子体波导和互连具有潜在影响。