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塔姆等离激元定向增强稀土纳米磷光体发射。

Tamm Plasmons Directionally Enhance Rare-Earth Nanophosphor Emission.

作者信息

Geng Dongling, Cabello-Olmo Elena, Lozano Gabriel, Míguez Hernán

机构信息

Institute of Materials Science of Seville, Consejo Superior de Investigaciones Científicas (CSIC)-Universidad de Sevilla (US), Américo Vespucio 49, 41092, Seville, Spain.

出版信息

ACS Photonics. 2019 Mar 20;6(3):634-641. doi: 10.1021/acsphotonics.8b01407. Epub 2019 Feb 14.

Abstract

Rare-earth-based phosphors are the materials on which current solid-state lighting technology is built. However, their large crystal size impedes the tuning, optimization, or manipulation of emitted light that can be achieved by their integration in nanophotonic architectures. Herein we demonstrate a hybrid plasmonic-photonic architecture capable of both channeling in a specific direction and enhancing by eight times the emission radiated by a macroscopically wide layer of nanophosphors. In order to do so, a slab of rare-earth-based nanocrystals is inserted between a dielectric multilayer and a metal film, following a rational design that optimizes the coupling of nanophosphor emission to collective modes sustained by the metal-dielectric system. Our approach is advantageous for the optimization of solid-state lighting systems.

摘要

基于稀土的磷光体是当前固态照明技术所依赖的材料。然而,它们较大的晶体尺寸阻碍了通过将其集成到纳米光子结构中所能实现的发射光的调谐、优化或操控。在此,我们展示了一种混合等离子体-光子结构,它既能在特定方向上引导光,又能将宏观上较宽的纳米磷光体层所辐射的发射光增强八倍。为了实现这一点,按照一种合理的设计,将一层基于稀土的纳米晶体插入到一个介电多层膜和一个金属膜之间,该设计优化了纳米磷光体发射与金属-介电系统所维持的集体模式之间的耦合。我们的方法对于固态照明系统的优化是有利的。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/8ca9/6488127/2032d9797c84/ph-2018-01407w_0001.jpg

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