Moon Byoung Hee, Bae Jung Jun, Han Gang Hee, Kim Hyun, Choi Homin, Lee Young Hee
Center for Integrated Nanostructure Physics , Institute for Basic Science (IBS) , Suwon 16419 , Republic of Korea.
Department of Energy Science , Sungkyunkwan University , Suwon 16419 , Republic of Korea.
ACS Nano. 2019 Jun 25;13(6):6631-6637. doi: 10.1021/acsnano.9b00755. Epub 2019 May 28.
Conductivity of the insulating phase increases generally at an elevated drain-source voltage due to the field-enhanced hopping or heating effect. Meanwhile, a transport mechanism governed by percolation in a low compensated semiconductor gives rise to the reduced conductivity at a low-field regime. Here, in addition to this behavior, we report the anomalous conductivity behavior to transform from a percolative metallic to an insulating phase at the low voltage regime in monolayer molybdenum disulfide (MoS). Percolation transport at low source-drain voltage is governed by inhomogeneously distributed potential in strongly interacting monolayer MoS with a substrate, distinct from the quantum phase transition in multilayer MoS. At a high source-drain voltage regime, the insulating phase is transformed further to a metallic phase, exhibiting multiphases of metallic-insulating-metallic transitions in monolayer MoS. These behaviors highlight MoS as a model system to study various classical and quantum transports as well as metal-insulator transition in two-dimensional systems.
由于场增强跳跃或热效应,绝缘相的电导率通常在漏源电压升高时增加。同时,在低补偿半导体中由渗流控制的传输机制导致在低场区域电导率降低。在此,除了这种行为之外,我们还报告了单层二硫化钼(MoS)在低电压区域从渗流金属相转变为绝缘相的异常导电行为。低源漏电压下的渗流传输由与衬底强相互作用的单层MoS中不均匀分布的电势控制,这与多层MoS中的量子相变不同。在高源漏电压区域,绝缘相进一步转变为金属相,在单层MoS中呈现金属 - 绝缘 - 金属转变的多相。这些行为突出了MoS作为研究二维系统中各种经典和量子传输以及金属 - 绝缘体转变的模型系统。