Semeniuk Maria, Yi Zhihui, Poursorkhabi Vida, Tjong Jimi, Jaffer Shaffiq, Lu Zheng-Hong, Sain Mohini
Centre for Biocomposites and Biomaterials Processing, Faculty of Forestry , University of Toronto , 33 Willcocks Street , Toronto , Ontario M5S 3B3 , Canada.
Department of Material Science and Engineering , University of Toronto , 184 College Street , Toronto , Ontario M5S 3A1 , Canada.
ACS Nano. 2019 Jun 25;13(6):6224-6255. doi: 10.1021/acsnano.9b00688. Epub 2019 Jun 4.
Over the span of the past decade, carbon dots (CDs) synthesized from renewable organic resources (organic CDs) have gathered a considerable amount of attention for their photoluminescent properties. This review will focus on organic CDs synthesized using clean chemistry and conventional synthetic chemistry from organic sources and their fluorescence mechanisms, such as quantum confinement effect and surface/edge defects, before outlining their performance in electronic applications, including organic photovoltaic devices, organic light-emitting devices, biosensors, supercapacitors, and batteries. The various organic resources and methods of organic CDs synthesis are briefly covered. Many challenges remain before the adoption of CDs can become widespread; their characterization, structure, functionality, and exact photoluminescent mechanism all require additional research. This review aims to summarize the current research outcomes and highlight the area where further research is needed to fully use these materials.
在过去十年中,由可再生有机资源合成的碳点(CDs,有机碳点)因其光致发光特性而备受关注。本综述将聚焦于通过清洁化学和传统合成化学从有机源合成的有机碳点及其荧光机制,如量子限域效应和表面/边缘缺陷,然后概述它们在电子应用中的性能,包括有机光伏器件、有机发光器件、生物传感器、超级电容器和电池。简要介绍了各种有机资源和有机碳点的合成方法。在碳点得到广泛应用之前,仍存在许多挑战;它们的表征、结构、功能以及确切的光致发光机制都需要进一步研究。本综述旨在总结当前的研究成果,并突出需要进一步研究以充分利用这些材料的领域。