Hermenau Jan, Brinker Sascha, Marciani Marco, Steinbrecher Manuel, Dos Santos Dias Manuel, Wiesendanger Roland, Lounis Samir, Wiebe Jens
Department of Physics, Hamburg University, 20355, Hamburg, Germany.
Peter Grünberg Institut and Institute for Advanced Simulation, Forschungszentrum Jülich & JARA, 52425, Jülich, Germany.
Nat Commun. 2019 Jun 12;10(1):2565. doi: 10.1038/s41467-019-10516-2.
Spins of single atoms adsorbed on substrates are promising building blocks for spintronics and quantum computation schemes. To process spin information and for increased magnetic stability, these spins have to be coupled to arrays. For a single atom, a high symmetry of the environment increases its spin stability. However, little is known about the role of the symmetry of the magnetic couplings in the arrays. Here, we study arrays of atomic spins coupled via Ruderman-Kittel-Kasuya-Yosida interaction, focusing on Dzyaloshinskii-Moriya and symmetric anisotropic exchange. We show that the high spin stability of a trimer can be remotely detected by a nearby atom, and how the Dzyaloshinskii-Moriya interaction leads to its destabilization. Adding more nearby atoms further destabilizes the trimer, due to a non-local effective transverse anisotropy originating in the symmetric anisotropic exchange. This transverse anisotropy can be quenched for highly symmetric structures, where the spin lifetime of the array increases drastically.
吸附在衬底上的单个原子的自旋是自旋电子学和量子计算方案中很有前景的构建模块。为了处理自旋信息并提高磁稳定性,这些自旋必须耦合到阵列中。对于单个原子,环境的高对称性会增加其自旋稳定性。然而,关于阵列中磁耦合对称性的作用却知之甚少。在这里,我们研究通过Ruderman-Kittel-Kasuya-Yosida相互作用耦合的原子自旋阵列,重点关注Dzyaloshinskii-Moriya和对称各向异性交换。我们表明,三聚体的高自旋稳定性可以被附近的原子远程检测到,以及Dzyaloshinskii-Moriya相互作用如何导致其失稳。由于对称各向异性交换产生的非局域有效横向各向异性,添加更多附近的原子会进一步使三聚体失稳。对于高度对称的结构,这种横向各向异性可以被消除,此时阵列的自旋寿命会急剧增加。