Institute for Energy, Environment and Sustainable Communities, University of Regina, Regina, S4S 0A2, Canada; MOE Key Laboratory of Resources and Environmental Systems Optimization, North China Electric Power University, Beijing, 102206, China.
Institute for Energy, Environment and Sustainable Communities, University of Regina, Regina, S4S 0A2, Canada.
Chemosphere. 2020 Apr;245:125545. doi: 10.1016/j.chemosphere.2019.125545. Epub 2019 Dec 6.
Ceramic water filter is suitable for low-income families and rural communities in developing countries to obtain safe drinking water because of its low cost and good performance. As an innovative effort, the ceramic disk filter coated with Ag/ZnO nanocomposites (AZ-CDF) was proposed in this study. The manufacture of AZ-CDFs was optimized by experiments based on the Box-Behnken design. The results of thermal field emission scanning electron microscopy (TFE-SEM) and very powerful elemental and structural probe employing radiation from a synchrotron (VESPERS) indicated that Ag/ZnO nanocomposites were mainly distributed on the upper surface of AZ-CDF. The antibacterial activity of AZ-CDF was investigated by detecting the variation of cell status and intracellular reactive oxygen species during a period of time using flow cytometry. Both non-photocatalytic and photocatalytic antibacterial activities of Ag/ZnO nanocomposite contributed to the bacterial reduction property of AZ-CDF. During filtration, the initial Escherichia coli (E. coli) concentration and illumination intensity also influenced the E. coli removal performance of AZ-CDF. When the light illumination intensity was 7000 Lux, AZ-CDF was appropriate to treat the water contaminated by E. coli concentration of less than 10 cfu/mL. Increasing illumination intensity resulted in the improvement of E. coli removal performance of AZ-CDF. It was concluded the main mechanisms for the E. coli removal of AZ-CDF were filtration, non-photocatalytic and photocatalytic antibacterial activities.
陶瓷水过滤器适合低收入家庭和发展中国家的农村社区使用,因为其成本低、性能好,可以获得安全的饮用水。作为一项创新努力,本研究提出了一种涂覆有 Ag/ZnO 纳米复合材料的陶瓷圆盘过滤器(AZ-CDF)。通过基于 Box-Behnken 设计的实验优化了 AZ-CDF 的制造。热场发射扫描电子显微镜(TFE-SEM)和非常强大的元素和结构探测仪(VESPERS)的结果表明,Ag/ZnO 纳米复合材料主要分布在 AZ-CDF 的上表面。通过使用流式细胞术检测一段时间内细胞状态和细胞内活性氧的变化来研究 AZ-CDF 的抗菌活性。Ag/ZnO 纳米复合材料的非光催化和光催化抗菌活性都有助于 AZ-CDF 的细菌减少特性。在过滤过程中,初始大肠杆菌(E. coli)浓度和光照强度也会影响 AZ-CDF 的大肠杆菌去除性能。当光照强度为 7000 Lux 时,AZ-CDF 适合处理大肠杆菌浓度低于 10 cfu/mL 的污染水。增加光照强度会提高 AZ-CDF 的大肠杆菌去除性能。研究结论为 AZ-CDF 去除大肠杆菌的主要机制是过滤、非光催化和光催化抗菌活性。