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具有石墨烯涂层纳米盘同二聚体的多频近场增强

Multi-frequency near-field enhancement with graphene-coated nano-disk homo-dimers.

作者信息

Raad Shiva Hayati, Atlasbaf Zahra, Zapata-Rodríguez Carlos J

出版信息

Opt Express. 2019 Dec 9;27(25):37012-37024. doi: 10.1364/OE.27.037012.

DOI:10.1364/OE.27.037012
PMID:31873471
Abstract

In this paper, a 3D sub-wavelength graphene-coated nano-disk dimer (GDD) is proposed for multi-frequency giant near-field enhancement. We observed that the dual-band operation originates from the excitation of hybridized localized surface plasmons on top and bottom faces of the disks along with the mutual coupling from the adjacent particle. Due to the sub-wavelength nature of the disks, the excited localized surface plasmons on the sidewalls are weak but they still can affect the dual operating bands. On the other hand, the strength and resonance frequency of the enhanced fields can be simply modulated by tuning the relative distances of 2D graphene disks on top and bottom faces. Adjustable dual-band performance is hardly attainable using simplified 2D graphene disks, however, it naturally comes out through modal hybridization in the subwavelength 3D structure containing multiple resonant units. Our suggested configuration has better optical properties than its noble metal counterparts because of its higher field enhancement and lower ohmic losses. Moreover, the electromagnetic response is reconfigurable by varying the bias voltage. The influence of graphene quality, chemical potential, and dimer gap size on the electric field enhancement and the resonance frequency of the surface plasmons are investigated, as well. To further improve its performance, a double negative metamaterial core is considered. This mechanism of the performance improvement by the core material is feasible thanks to the 3D nature of the structure. Two possible applications of the presented design are in Surface-Enhanced Raman Spectroscopy (SERS) and optical absorbers.

摘要

本文提出了一种用于多频巨近场增强的三维亚波长石墨烯包覆纳米盘二聚体(GDD)。我们观察到,双频操作源于盘的顶面和底面杂化局域表面等离子体激元的激发以及相邻粒子的相互耦合。由于盘的亚波长特性,侧壁上激发的局域表面等离子体激元较弱,但它们仍会影响双工作频段。另一方面,通过调整顶面和底面二维石墨烯盘的相对距离,可以简单地调制增强场的强度和共振频率。然而,使用简化的二维石墨烯盘很难实现可调双频性能,而在包含多个共振单元的亚波长三维结构中,通过模式杂化自然会出现这种性能。由于其更高的场增强和更低的欧姆损耗,我们提出的结构比其贵金属对应物具有更好的光学性质。此外,通过改变偏置电压,电磁响应是可重构的。还研究了石墨烯质量、化学势和二聚体间隙尺寸对电场增强和表面等离子体激元共振频率的影响。为了进一步提高其性能,考虑了一种双负超材料核心。由于结构的三维性质,核心材料改善性能的这种机制是可行的。所提出设计的两个可能应用是在表面增强拉曼光谱(SERS)和光吸收器中。

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