State Key Laboratory of Cryospheric Science, Chinese Academy of Sciences (CAS), Northwest Institute of Eco-Environment and Resources, CAS, DongGangXi Road, Chengguan District, Lanzhou, 730000, People's Republic of China.
CAS Center for Excellence in Tibetan Plateau Earth Sciences, Beijing, 100101, China.
Environ Sci Pollut Res Int. 2020 Apr;27(10):10617-10628. doi: 10.1007/s11356-020-07618-6. Epub 2020 Jan 15.
Total suspended particles (TSP) were collected in Lumbini from April 2013 to March 2016 to better understand the characteristics of carbonaceous aerosol (CA) concentrations, compositions and sources and their light absorption properties in rural region of severe polluted Indo-Gangetic Plain (IGP). Extremely high TSP (203.9 ± 109.6 μg m), organic carbon (OC 32.1 ± 21.7 μg m), elemental carbon (EC 6.44 ± 3.17 μg m) concentrations were observed in Lumbini particularly during winter and post-monsoon seasons, reflecting the combined influences of emission sources and weather conditions. SO (7.34 ± 4.39 μg m) and Ca (5.46 ± 5.20 μg m) were the most dominant anion and cation in TSP. These components were comparable to those observed in urban areas in South and East Asia but significantly higher than those in remote regions over the Himalayas and Tibetan Plateau, suggesting severe air pollution in the study region. Various combustion activities including industry, vehicle emission, and biomass burning are the main reasons for high pollutant concentrations. The variation of OC/EC ratio further suggested that biomass such as agro-residue burning contributed a lot for CA, particularly during the non-monsoon season. The average mass absorption cross-section of EC (MAC) and water-soluble organic carbon (MAC) were 7.58 ± 3.39 and 1.52 ± 0.41 m g, respectively, indicating that CA in Lumbini was mainly affected by local emissions. Increased biomass burning decreased MAC; whereas, it could result in high MAC during the non-monsoon season. Furthermore, dust is one important factor causing higher MAC during the pre-monsoon season.
从 2013 年 4 月到 2016 年 3 月,在蓝毗尼采集了总悬浮颗粒物(TSP),以便更好地了解碳质气溶胶(CA)浓度、组成和来源的特征,以及它们在严重污染的印度-恒河平原(IGP)农村地区的光吸收特性。在蓝毗尼,TSP(203.9±109.6μg/m)、有机碳(OC 32.1±21.7μg/m)、元素碳(EC 6.44±3.17μg/m)浓度极高,特别是在冬季和后季风季节,这反映了排放源和天气条件的综合影响。SO(7.34±4.39μg/m)和 Ca(5.46±5.20μg/m)是 TSP 中最主要的阴离子和阳离子。这些成分与南亚和东亚城市地区观察到的成分相当,但明显高于喜马拉雅山和青藏高原偏远地区的成分,表明研究地区空气污染严重。各种燃烧活动,包括工业、车辆排放和生物质燃烧,是污染物浓度高的主要原因。OC/EC 比值的变化进一步表明,生物质(如农业残留物燃烧)是 CA 的主要来源,特别是在非季风季节。EC 的质量吸收截面(MAC)和水溶性有机碳(MAC)的平均值分别为 7.58±3.39 和 1.52±0.41 m/g,表明蓝毗尼的 CA 主要受当地排放的影响。生物质燃烧的增加会降低 MAC;然而,在非季风季节,它可能导致 MAC 升高。此外,灰尘是前季风季节导致更高 MAC 的一个重要因素。