Environmental Engineering , University of Illinois Urbana-Champaign , Urbana , Illinois 61801 , United States.
Institute of Tibetan Plateau Research, Chinese Academy of Sciences , Center for Excellence in Tibetan Plateau Earth Sciences , Beijing 100101 , China.
Environ Sci Technol. 2019 Mar 19;53(6):3306-3314. doi: 10.1021/acs.est.8b05199. Epub 2019 Mar 11.
Traditional biomass stoves are a major global contributor to emissions that impact climate change and health. This paper reports emission factors of particulate matter (PM), carbon monoxide (CO), organic carbon (OC), black carbon (EC), optical absorption, and scattering from 46 South Asian, 48 Tibetan, and 4 Ugandan stoves. These measurements plus a literature review provide insight into the robustness of emission factors used in emission inventories. Tibetan dung stoves produced high average PM emission factors (23 and 43 gkg for chimney and open stoves) with low average EC (0.3 and 0.7 gkg, respectively). Comparatively, PM from South Asian stoves (7 gkg) was in the range of previous measurements and near values used in inventories. EC emission factors varied between stoves and fuels ( p < 0.001), without corresponding differences in absorption; stoves that produced little EC, produced enough brown carbon to have about the same absorption as stoves with high EC emissions. In Tibetan dung stoves, for example, OC contributed over 20% of the absorption. Overall, EC emission factors were not correlated with PM and were constrained to low values, relative to PM, over a wide range of combustion conditions. The average measured EC emission factor (1 gkg), was near current inventory estimates.
传统生物质炉灶是全球主要的排放源之一,这些排放物对气候变化和健康都有影响。本文报告了来自 46 个南亚、48 个西藏和 4 个乌干达炉灶的颗粒物(PM)、一氧化碳(CO)、有机碳(OC)、黑碳(EC)、光吸收和散射的排放因子。这些测量结果加上文献综述,深入了解了排放清单中使用的排放因子的稳健性。西藏牛粪炉灶产生的 PM 排放因子较高(烟囱和开放式炉灶分别为 23 和 43 gkg),而 EC 平均排放量较低(分别为 0.3 和 0.7 gkg)。相比之下,南亚炉灶的 PM(7 gkg)处于先前测量值的范围内,与清单中使用的值相近。EC 排放因子因炉灶和燃料而异(p < 0.001),但吸收没有相应差异;产生少量 EC 的炉灶产生的棕碳足以使其吸收与 EC 排放量高的炉灶相当。例如,在西藏牛粪炉灶中,OC 对吸收的贡献超过 20%。总的来说,EC 排放因子与 PM 不相关,并且在广泛的燃烧条件下,相对于 PM 受到限制,处于低值。平均实测 EC 排放因子(1 gkg)接近当前清单估计值。