Van Nguyen Khoe, Chang Yia-Chung
Research Center for Applied Sciences, Academia Sinica, Taipei 115, Taiwan.
Phys Chem Chem Phys. 2020 Feb 21;22(7):3999-4009. doi: 10.1039/c9cp05740d. Epub 2020 Feb 5.
The in-plane acoustic phonon scattering in graphene is solved by considering fully inelastic acoustic phonon scatterings in two-dimensional (2D) Dirac materials for a large range of temperatures (T) and chemical potentials (μ). Rigorous analytical solutions and symmetry properties of Fermionic and Bosonic functions are obtained. We illustrate how doping alters the temperature dependence of acoustic phonon scattering rates. It is shown that the quasi-elastic and ansatz equations previously derived for acoustic phonon scatterings in graphene are limiting cases of the inelastic-scattering equations derived here. For heavily-doped graphene, we found that the high-T behavior of resistivity is better described by ρ(T,μ) ∝T(1 -ζμ/3(kT)) rather than a linear T behavior, and in the low T regime we found τ∝ (kT) but with a different prefactor (i.e.∼3 times smaller) in comparison with the existing quasi-elastic expressions. Furthermore, we found a simple analytic "semi-inelastic" expression of the form τ∝ (kT)/(1 + cT) which matches nearly perfectly with the full inelastic results for any temperature up to 500 K and μ up to 1 eV. Our simple analytical results agree well with previous first-principles studies and available experimental data. Moreover, we obtain an analytical form for the acoustic gauge field . Our analyses pave a way for investigating scatterings between electrons and other fundamental excitations with linear dispersion relation in 2D Dirac material-based heterostructures such as bogolon-mediated electron scattering in graphene-based hybrid Bose-Fermi systems.
通过考虑二维(2D)狄拉克材料在大范围温度(T)和化学势(μ)下的完全非弹性声子散射,求解了石墨烯中的面内声子散射。得到了费米子和玻色子函数的严格解析解及对称性质。我们阐述了掺杂如何改变声子散射率的温度依赖性。结果表明,先前为石墨烯中的声子散射推导的准弹性和假设方程是此处推导的非弹性散射方程的极限情况。对于重掺杂石墨烯,我们发现电阻率的高温行为用ρ(T,μ) ∝T(1 -ζμ/3(kT)) 能更好地描述,而非线性T行为,并且在低温区我们发现τ∝ (kT) ,但与现有的准弹性表达式相比,其前置因子不同(即小约3倍)。此外,我们发现了一个简单的解析“半非弹性”表达式,形式为τ∝ (kT)/(1 + cT) ,在高达500 K的任何温度和高达1 eV的μ下,它与完全非弹性结果几乎完美匹配。我们简单的解析结果与先前的第一性原理研究和现有实验数据吻合良好。此外,我们得到了声学规范场的解析形式。我们的分析为研究二维狄拉克材料基异质结构中电子与具有线性色散关系的其他基本激发之间的散射铺平了道路,例如基于石墨烯的混合玻色 - 费米系统中玻戈龙介导的电子散射。