Do Seung-Hwan, Lee C H, Kihara T, Choi Y S, Yoon Sungwon, Kim Kangwon, Cheong Hyeonsik, Chen Wei-Tin, Chou Fangcheng, Nojiri H, Choi Kwang-Yong
Department of Physics, Chung-Ang University, Seoul 06974, Republic of Korea.
Institute for Materials Research, Tohoku University, Katahira 2-1-1, Sendai 980-8577, Japan.
Phys Rev Lett. 2020 Jan 31;124(4):047204. doi: 10.1103/PhysRevLett.124.047204.
dc and ac magnetic susceptibility, magnetization, specific heat, and Raman scattering measurements are combined to probe low-lying spin excitations in α-Ru_{1-x}Ir_{x}Cl_{3} (x≈0.2), which realizes a disordered spin liquid. At intermediate energies (ℏω>3 meV), Raman spectroscopy evidences linearly ω-dependent Majorana-like excitations, obeying Fermi statistics. This points to robustness of a Kitaev paramagnetic state under spin vacancies. At low energies below 3 meV, we observe power-law dependences and quantum-critical-like scalings of the thermodynamic quantities, implying the presence of a weakly divergent low-energy density of states. This scaling phenomenology is interpreted in terms of the random hoppings of Majorana fermions. Our results demonstrate an emergent hierarchy of spin excitations in a diluted Kitaev honeycomb system subject to spin vacancies and bond randomness.
直流和交流磁化率、磁化强度、比热以及拉曼散射测量相结合,用于探测α-Ru₁₋ₓIrₓCl₃(x≈0.2)中的低能自旋激发,该材料实现了无序自旋液体。在中等能量(ℏω>3 meV)下,拉曼光谱证明了线性ω依赖的类马约拉纳激发,遵循费米统计。这表明在自旋空位下基泰夫顺磁态的稳健性。在低于3 meV的低能量下,我们观察到热力学量的幂律依赖关系和类量子临界标度,这意味着存在弱发散的低能态密度。这种标度现象学是根据马约拉纳费米子的随机跳跃来解释的。我们的结果表明,在存在自旋空位和键无序的稀释基泰夫蜂窝系统中,自旋激发出现了层次结构。