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A New Composite Structure of PEDOT/PSS: Macro-Separated Layers by a Polyelectrolyte Brush.

作者信息

Yasumoro Keita, Fujita Yushi, Arimatsu Hideki, Fujima Takuya

机构信息

Department of Mechanical Engineering, Tokyo City University, Tokyo 158-8557, Japan.

Advanced Research Laboratories, Tokyo City University, Tokyo 158-0082, Japan.

出版信息

Polymers (Basel). 2020 Feb 16;12(2):456. doi: 10.3390/polym12020456.

DOI:10.3390/polym12020456
PMID:32079081
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC7077716/
Abstract

Polyethylene dioxythiophene and polyethylene sulfonic acid (PEDOT/PSS) composite is gathering attention as an organic transparent conductive film material. However, it requires a core-shell structure in which conductive PEDOT is covered with insulating PSS. Providing film formability and a carrier to PEDOT, the PSS shell hinders carrier conduction as an insulating barrier. In this study, we realized that creating a macro-separated PEDOT/PSS composite by using a polyelectrolyte brush substrate and in-situ PEDOT polymerization without the PSS barrier increases durability and conductivity in comparison with commercially available PEDOT/PSS film, achieving a conductivity of 5000-6000 S/cm.

摘要
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/19b4/7077716/e0957f1bf23d/polymers-12-00456-g006.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/19b4/7077716/bc022f3563e2/polymers-12-00456-g001.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/19b4/7077716/05ce2d8848b1/polymers-12-00456-g002.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/19b4/7077716/ed3449af7637/polymers-12-00456-g003.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/19b4/7077716/a6db732849c9/polymers-12-00456-g004.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/19b4/7077716/9489d9d1275b/polymers-12-00456-g005.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/19b4/7077716/e0957f1bf23d/polymers-12-00456-g006.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/19b4/7077716/bc022f3563e2/polymers-12-00456-g001.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/19b4/7077716/05ce2d8848b1/polymers-12-00456-g002.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/19b4/7077716/ed3449af7637/polymers-12-00456-g003.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/19b4/7077716/a6db732849c9/polymers-12-00456-g004.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/19b4/7077716/9489d9d1275b/polymers-12-00456-g005.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/19b4/7077716/e0957f1bf23d/polymers-12-00456-g006.jpg

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本文引用的文献

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Anal Chem. 2017 Mar 21;89(6):3508-3516. doi: 10.1021/acs.analchem.6b04625. Epub 2017 Feb 27.
2
Simultaneously Enhancing the Cohesion and Electrical Conductivity of PEDOT:PSS Conductive Polymer Films using DMSO Additives.使用二甲基亚砜添加剂同时增强聚（3,4-乙撑二氧噻吩）：聚苯乙烯磺酸盐导电聚合物薄膜的内聚力和导电性
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对甲苯磺酸在具有大塞贝克系数的聚（3,4-乙撑二氧噻吩）：对甲苯磺酸的电导率中的双重作用
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Poly(3,4-ethylenedioxythiophene) Electrosynthesis in the Presence of Mixtures of Flexible-Chain and Rigid-Chain Polyelectrolytes.在柔性链和刚性链聚电解质混合物存在下的聚（3,4-亚乙基二氧噻吩）电合成
Polymers (Basel). 2021 Nov 9;13(22):3866. doi: 10.3390/polym13223866.
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First-Principle Study on p-n Control of PEDOT-Based Thermoelectric Materials by PTSA Doping.基于PTSA掺杂的PEDOT基热电材料p-n控制的第一性原理研究
Polymers (Basel). 2021 Oct 13;13(20):3518. doi: 10.3390/polym13203518.
Hierarchical nanoporous glass with antireflectivity and superhydrophilicity by one-pot etching.
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