Department of Biochemistry, University of Wisconsin, Madison, Wisconsin, United States.
Protein Sci. 2020 May;29(5):1148-1159. doi: 10.1002/pro.3843. Epub 2020 Mar 4.
The exciting discovery of the giant DNA Mimivirus in 2003 challenged the conventional description of viruses in a radical way, and since then, dozens of additional giant viruses have been identified. It has now been demonstrated that the Mimivirus genome encodes for the two enzymes required for the production of the unusual sugar 4-amino-4,6-dideoxy-d-glucose, namely a 4,6-dehydratase and an aminotransferase. In light of our long-standing interest in the bacterial 4,6-dehydratases and in unusual sugars in general, we conducted a combined structural and functional analysis of the Mimivirus 4,6-dehydratase referred to as R141. For this investigation, the three-dimensional X-ray structure of R141 was determined to 2.05 Å resolution and refined to an R-factor of 18.3%. The overall fold of R141 places it into the short-chain dehydrogenase/reductase (SDR) superfamily of proteins. Whereas its molecular architecture is similar to that observed for the bacterial 4,6-dehydratases, there are two key regions where the polypeptide chain adopts different conformations. In particular, the conserved tyrosine that has been implicated as a catalytic acid or base in SDR superfamily members is splayed away from the active site by nearly 12 Å, thereby suggesting that a major conformational change must occur upon substrate binding. In addition to the structural analysis, the kinetic parameters for R141 using either dTDP-d-glucose or UDP-d-glucose as substrates were determined. Contrary to a previous report, R141 demonstrates nearly identical catalytic efficiency with either nucleotide-linked sugar. The data presented herein represent the first three-dimensional model for a viral 4,6-dehydratase and thus expands our understanding of these fascinating enzymes.
2003 年,巨型 DNA 拟病毒的惊人发现从根本上挑战了病毒的传统描述方式,此后,又发现了数十种额外的巨型病毒。现在已经证明,拟病毒基因组编码了产生不寻常糖 4-氨基-4,6-二脱氧-d-葡萄糖所需的两种酶,即 4,6-脱水酶和氨基转移酶。鉴于我们对细菌 4,6-脱水酶和一般不寻常糖的长期兴趣,我们对被称为 R141 的拟病毒 4,6-脱水酶进行了结构和功能的综合分析。为此,我们确定了 R141 的三维 X 射线结构,分辨率为 2.05 Å,并将其精炼至 R 因子为 18.3%。R141 的整体折叠将其归入短链脱氢酶/还原酶 (SDR) 超家族蛋白。尽管其分子结构与细菌 4,6-脱水酶相似,但在两个关键区域,多肽链采用了不同的构象。特别是,保守的酪氨酸被认为是 SDR 超家族成员中的催化酸或碱基,其与活性位点的距离相差近 12 Å,这表明在底物结合时必须发生主要的构象变化。除了结构分析外,还使用 dTDP-d-葡萄糖或 UDP-d-葡萄糖作为底物确定了 R141 的动力学参数。与之前的报道相反,R141 对核苷酸连接的糖表现出几乎相同的催化效率。本文提供的数据代表了第一个病毒 4,6-脱水酶的三维模型,从而扩展了我们对这些迷人酶的理解。