Experimentalphysik VI, Center for Electronic Correlations and Magnetism, University of Augsburg, 86159 Augsburg, Germany.
Institute of Crystallography, RWTH Aachen University and Jülich Centre for Neutron Science (JCNS) at Heinz Maier-Leibnitz Zentrum (MLZ), D-85747 Garching, Germany.
Science. 2020 Mar 13;367(6483):1218-1223. doi: 10.1126/science.aaw1666.
Spin ices are exotic phases of matter characterized by frustrated spins obeying local "ice rules," in analogy with the electric dipoles in water ice. In two dimensions, one can similarly define ice rules for in-plane Ising-like spins arranged on a kagome lattice. These ice rules require each triangle plaquette to have a single monopole and can lead to different types of orders and excitations. Using experimental and theoretical approaches including magnetometry, thermodynamic measurements, neutron scattering, and Monte Carlo simulations, we establish HoAgGe as a crystalline (i.e., nonartificial) system that realizes the kagome spin ice state. The system features a variety of partially and fully ordered states and a sequence of field-induced phases at low temperatures, all consistent with the kagome ice rule.
自旋冰是一种奇特的物质相,其特征是受局域“冰规则”约束的 frustrated spins,类似于水冰中的电偶极子。在二维空间中,人们可以类似地为 kagome 晶格上排列的面内类 Ising 自旋定义冰规则。这些冰规则要求每个三角形 plaquette 只有一个单极子,并可以导致不同类型的序和激发。通过使用包括磁强计、热力学测量、中子散射和蒙特卡罗模拟在内的实验和理论方法,我们确立了 HoAgGe 是一种实现 kagome 自旋冰状态的晶体(即非人为)系统。该系统具有多种部分和完全有序的状态以及一系列低温下的场诱导相,所有这些都与 kagome 冰规则一致。