Zheng Guoxin, Zhu Yuan, Chen Kuan-Wen, Kang Byungmin, Zhang Dechen, Jenkins Kaila, Chan Aaron, Zeng Zhenyuan, Xu Aini, Valenzuela Oscar A, Blawat Joanna, Singleton John, Li Shiliang, Lee Patrick A, Li Lu
Department of Physics, University of Michigan, Ann Arbor, MI 48109.
Department of Physics, Massachusetts Institute of Technology, Cambridge, MA 02139.
Proc Natl Acad Sci U S A. 2025 Feb 4;122(5):e2421390122. doi: 10.1073/pnas.2421390122. Epub 2025 Jan 31.
In metals, electrons in a magnetic field undergo cyclotron motion, leading to oscillations in physical properties called quantum oscillations. This phenomenon has never been seen in a robust insulator because there are no mobile electrons. We report an exception to this rule. We study a Mott insulator on a kagome lattice which does not order magnetically down to milli-Kelvin temperatures despite antiferromagnetic interactions. We observe a plateau at magnetization equal to [Formula: see text] Bohr magneton per magnetic ion, accompanied by oscillations in the magnetic torque, reminiscent of quantum oscillations in metals. The temperature dependence obeys Fermi distribution. These phenomena are consistent with a quantum spin liquid state whose excitations are fermionic spinons with a Dirac-like spectrum coupled to an emergent gauge field.
在金属中,处于磁场中的电子会进行回旋运动,从而导致被称为量子振荡的物理性质发生振荡。这种现象在坚固的绝缘体中从未被观察到,因为其中不存在可移动的电子。我们报告了这一规则的一个例外情况。我们研究了一种位于 Kagome 晶格上的莫特绝缘体,尽管存在反铁磁相互作用,但在低至毫开尔文温度下它都不会发生磁有序。我们观察到磁化强度达到每个磁性离子[公式:见原文]玻尔磁子处出现一个平台,同时伴随着磁转矩的振荡,这让人联想到金属中的量子振荡。其温度依赖性符合费米分布。这些现象与一种量子自旋液体状态相一致,该状态的激发是具有类狄拉克谱的费米子自旋子,并与一个涌现的规范场耦合。