Makarenko Ksenia S, Hoang Thanh Xuan, Duffin Thorin J, Radulescu Andreea, Kalathingal Vijith, Lezec Henri J, Chu Hong-Son, Nijhuis Christian A
Department of Chemistry National University of Singapore 3 Science Drive Singapore 117543 Singapore.
Department of Electronics and Photonics Institute of High Performance Computing ASTAR (Agency for Science, Technology and Research) 1 Fusionopolis Way, #16-16 Connexis Singapore 138632 Singapore.
Adv Sci (Weinh). 2020 Feb 22;7(8):1900291. doi: 10.1002/advs.201900291. eCollection 2020 Apr.
Surface plasmon polaritons (SPPs) are viable candidates for integration into on-chip nano-circuitry that allow access to high data bandwidths and low energy consumption. Metal-insulator-metal tunneling junctions (MIM-TJs) have recently been shown to excite and detect SPPs electrically; however, experimentally measured efficiencies and outcoupling mechanisms are not fully understood. It is shown that the MIM-TJ cavity SPP mode (MIM-SPP) can outcouple via three pathways to i) photons via scattering of MIM-SPP at the MIM-TJ interfaces, ii) SPPs at the metal-dielectric interfaces (bound-SPPs) by mode coupling through the electrodes, and iii) photons and bound-SPP modes by mode coupling at the MIM-TJ edges. It is also shown that, for Al-AlO -Cr-Au MIM-TJs on glass, the MIM-SPP mode outcouples efficiently to bound-SPPs through either electrode (pathway 2); this outcoupling pathway can be selectively turned on and off by changing the respective electrode thickness. Outcoupling at the MIM-TJ edges (pathway 3) is efficient and sensitive to the edge topography, whereas most light emission originates from roughness-induced scattering of the MIM-SPP mode (pathway 1). Using an arbitrary roughness profile, it is demonstrated that various roughness facets can raise MIM-SPP outcoupling efficiencies to 0.62%. These results pave the way for understanding the topographical parameters needed to develop CMOS-compatible plasmonic circuitry elements.
表面等离激元极化子(SPPs)是集成到片上纳米电路中的可行候选者,可实现高数据带宽和低能耗。金属 - 绝缘体 - 金属隧道结(MIM - TJs)最近已被证明能够电激发和检测SPPs;然而,实验测量的效率和外耦合机制尚未完全理解。研究表明,MIM - TJ腔表面等离激元极化子模式(MIM - SPP)可以通过三种途径向外耦合:i)通过MIM - SPP在MIM - TJ界面处的散射产生光子;ii)通过电极的模式耦合在金属 - 电介质界面处产生表面等离激元极化子(束缚SPPs);iii)通过MIM - TJ边缘处的模式耦合产生光子和束缚SPP模式。研究还表明,对于玻璃上的Al - AlO - Cr - Au MIM - TJs,MIM - SPP模式通过任一电极有效地向外耦合到束缚SPPs(途径2);通过改变相应电极的厚度,可以选择性地打开和关闭这种外耦合途径。MIM - TJ边缘处的外耦合(途径3)效率高且对边缘形貌敏感,而大多数光发射源于MIM - SPP模式的粗糙度诱导散射(途径1)。使用任意粗糙度轮廓,证明各种粗糙度面可以将MIM - SPP外耦合效率提高到0.62%。这些结果为理解开发与CMOS兼容的等离子体电路元件所需的形貌参数铺平了道路。