Tiguntseva Ekaterina, Koshelev Kirill, Furasova Aleksandra, Tonkaev Pavel, Mikhailovskii Vladimir, Ushakova Elena V, Baranov Denis G, Shegai Timur, Zakhidov Anvar A, Kivshar Yuri, Makarov Sergey V
Department of Physics and Engineering, ITMO University, Saint Petersburg 197101, Russia.
Nonlinear Physics Center, Australian National University, Canberra, ACT 2601, Australia.
ACS Nano. 2020 Jul 28;14(7):8149-8156. doi: 10.1021/acsnano.0c01468. Epub 2020 Jun 8.
Subwavelength particles supporting Mie resonances underpin a strategy in nanophotonics for efficient control and manipulation of light by employing both an electric and a magnetic optically induced multipolar resonant response. Here, we demonstrate that monolithic dielectric nanoparticles made of CsPbBr halide perovskites can exhibit both efficient Mie-resonant lasing and structural coloring in the visible and near-IR frequency ranges. We employ a simple chemical synthesis with nearly epitaxial quality for fabricating subwavelength cubes with high optical gain and demonstrate single-mode lasing governed by the Mie resonances from nanocubes as small as 310 nm by the side length. These active nanoantennas represent the most compact room-temperature nonplasmonic nanolasers demonstrated until now.
支持米氏共振的亚波长粒子是纳米光子学中一种通过利用电和磁光学诱导多极共振响应来有效控制和操纵光的策略的基础。在此,我们证明由CsPbBr卤化物钙钛矿制成的单片介电纳米粒子在可见光和近红外频率范围内既能表现出高效的米氏共振激光发射,又能呈现结构色。我们采用一种具有近乎外延质量的简单化学合成方法来制造具有高光学增益的亚波长立方体,并证明边长小至310 nm的纳米立方体的米氏共振可控制单模激光发射。这些有源纳米天线是迄今为止所展示的最紧凑的室温非等离子体纳米激光器。