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由于晶格诱导的多极耦合,对称范德瓦尔斯异质结构超表面中的激光效应。

Lasing Effect in Symmetrical van der Waals Heterostructured Metasurfaces Due to Lattice-Induced Multipole Coupling.

作者信息

Prokhorov Alexei V, Gubin Mikhail Yu, Shesterikov Alexander V, Arsenin Aleksey V, Volkov Valentyn S, Evlyukhin Andrey B

机构信息

Emerging Technologies Research Center, XPANCEO, Dubai 00000, United Arab Emirates.

Institute of Quantum Optics, Leibniz Universität Hannover, Hannover 30167, Germany.

出版信息

Nano Lett. 2023 Dec 13;23(23):11105-11111. doi: 10.1021/acs.nanolett.3c03522. Epub 2023 Nov 29.

Abstract

New practical ways to reach the lasing effect in symmetrical metasurfaces have been developed and theoretically demonstrated. Our approach is based on excitation of the resonance of an octupole quasi-trapped mode (OQTM) in heterostructured symmetrical metasurfaces composed of monolithic disk-shaped van der Waals meta-atoms featured by thin photoluminescent layers and placed on a substrate. We revealed that the coincidence of the photoluminescence spectrum maximum of these layers with the wavelength of high-quality OQTM resonance leads to the lasing effect. Based on the solution of laser rate equations and direct full-wave simulation, it was shown that lasing is normally oriented to the metasurface plane and occurs from the entire area of metasurface consisting of MoS/hBN/MoTe disks with line width of generated emission of only about 1.4 nm near the wavelength 1140 nm. This opens up new practical possibilities for creating surface emitting laser devices in subwavelength material systems.

摘要

已开发并从理论上证明了在对称超表面中实现激光效应的新实用方法。我们的方法基于在由具有薄光致发光层且放置在衬底上的整体盘状范德华元原子组成的异质结构对称超表面中激发八极准捕获模式(OQTM)的共振。我们发现这些层的光致发光光谱最大值与高质量OQTM共振波长的重合导致了激光效应。基于激光速率方程的解和直接全波模拟,结果表明激光通常垂直于超表面平面,并且发生在由MoS/hBN/MoTe盘组成的超表面的整个区域,在波长1140nm附近产生的发射线宽仅约1.4nm。这为在亚波长材料系统中制造表面发射激光器件开辟了新的实际可能性。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/36dd/10880088/b96917e3efc9/nl3c03522_0001.jpg

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