Lorenz Malte, Weber Alfred P, Baune Michael, Thöming Jorg, Pesch Georg R
Faculty of Production Engineering, Chemical Process Engineering (CVT), University of Bremen, Bremen, Germany.
Institute of Particle Technology, Clausthal University of Technology, Clausthal-Zellerfeld, Germany.
Sci Rep. 2020 Jun 30;10(1):10617. doi: 10.1038/s41598-020-67628-9.
The possibilities and limitations using dielectrophoresis (DEP) for the dry classification of spherical aerosol particles was evaluated at low concentrations in a theoretical study. For an instrument with the geometry of concentric cylinders (similar to cylindrical DMA), the dependencies of target particle diameter [Formula: see text], resolution, and yield of the DEP classification on residence time, applied electric field strength, and pressure of the carrier gas were investigated. Further, the diffusion influence on the classification was considered. It was found that [Formula: see text] scales with the mean gas flow velocity [Formula: see text], classifier length L, and electric field strength E as [Formula: see text]. The resolution of the classification depends on the particle diameter and scales proportionally to [Formula: see text]. It is constrained by the flow ratio [Formula: see text] (i.e., sheath gas to aerosol flow), electrode diameters, and applied electric field strength. The classification yield increases with the ratio of the width of the extended outlet slit [Formula: see text] to the diffusion induced broadening [Formula: see text]. As expected, resolution and yield exhibit opposite dependencies on [Formula: see text]. Our simulations show that DEP classification can principally cover a highly interesting particle size range from 100 nm to [Formula: see text] while being directly particle size-selective and particle charge independent.
在一项理论研究中,评估了在低浓度下使用介电泳(DEP)对球形气溶胶颗粒进行干式分类的可能性和局限性。对于具有同心圆柱几何结构的仪器(类似于圆柱形微分迁移率分析仪),研究了目标粒径[公式:见原文]、分辨率以及DEP分类的产率对停留时间、施加的电场强度和载气压力的依赖性。此外,还考虑了扩散对分类的影响。研究发现,[公式:见原文]与平均气体流速[公式:见原文]、分级器长度L和电场强度E成比例,比例关系为[公式:见原文]。分类的分辨率取决于颗粒直径,并与[公式:见原文]成比例。它受到流量比[公式:见原文](即鞘气与气溶胶流量之比)、电极直径和施加的电场强度的限制。分类产率随着扩展出口狭缝宽度[公式:见原文]与扩散诱导展宽[公式:见原文]的比值增加而增加。正如预期的那样,分辨率和产率对[公式:见原文]呈现相反的依赖性。我们的模拟表明,DEP分类原则上可以覆盖从100纳米到[公式:见原文]的非常有趣的粒径范围,同时具有直接的粒径选择性且与颗粒电荷无关。