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飞秒激光在由X射线自由电子激光辐射探测的胶体晶体中产生周期性等离子体。

Femtosecond laser produced periodic plasma in a colloidal crystal probed by XFEL radiation.

作者信息

Mukharamova Nastasia, Lazarev Sergey, Meijer Janne-Mieke, Gorobtsov Oleg Yu, Singer Andrej, Chollet Matthieu, Bussmann Michael, Dzhigaev Dmitry, Feng Yiping, Garten Marco, Huebl Axel, Kluge Thomas, Kurta Ruslan P, Lipp Vladimir, Santra Robin, Sikorski Marcin, Song Sanghoon, Williams Garth, Zhu Diling, Ziaja-Motyka Beata, Cowan Thomas E, Petukhov Andrei V, Vartanyants Ivan A

机构信息

Deutsches Elektronen-Synchrotron DESY, Notkestraße 85, D-22607, Hamburg, Germany.

National Research Tomsk Polytechnic University (TPU), pr. Lenina 30, 634050, Tomsk, Russia.

出版信息

Sci Rep. 2020 Jul 1;10(1):10780. doi: 10.1038/s41598-020-67214-z.

DOI:10.1038/s41598-020-67214-z
PMID:
32612095
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC7329833/
Abstract

With the rapid development of short-pulse intense laser sources, studies of matter under extreme irradiation conditions enter further unexplored regimes. In addition, an application of X-ray Free-Electron Lasers (XFELs) delivering intense femtosecond X-ray pulses, allows to investigate sample evolution in IR pump - X-ray probe experiments with an unprecedented time resolution. Here we present a detailed study of the periodic plasma created from the colloidal crystal. Both experimental data and theory modeling show that the periodicity in the sample survives to a large extent the extreme excitation and shock wave propagation inside the colloidal crystal. This feature enables probing the excited crystal, using the powerful Bragg peak analysis, in contrast to the conventional studies of dense plasma created from bulk samples for which probing with Bragg diffraction technique is not possible. X-ray diffraction measurements of excited colloidal crystals may then lead towards a better understanding of matter phase transitions under extreme irradiation conditions.

摘要

随着短脉冲强激光源的迅速发展,对极端辐照条件下物质的研究进入了进一步未探索的领域。此外,应用产生强飞秒X射线脉冲的X射线自由电子激光器(XFEL),使得在红外泵浦-X射线探测实验中以前所未有的时间分辨率研究样品演化成为可能。在此,我们对由胶体晶体产生的周期性等离子体进行了详细研究。实验数据和理论建模均表明,样品中的周期性在很大程度上能经受住胶体晶体内的极端激发和冲击波传播。与对块状样品产生的稠密等离子体的传统研究不同,后者无法用布拉格衍射技术进行探测,而这一特性使得利用强大的布拉格峰分析来探测受激晶体成为可能。对受激胶体晶体的X射线衍射测量可能会有助于更好地理解极端辐照条件下的物质相变。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/db8a/7329833/b72e15ab1b25/41598_2020_67214_Fig5_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/db8a/7329833/f629695a1134/41598_2020_67214_Fig1_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/db8a/7329833/a73d0ea259c2/41598_2020_67214_Fig2_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/db8a/7329833/8cac386754fc/41598_2020_67214_Fig3_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/db8a/7329833/5958e46b735c/41598_2020_67214_Fig4_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/db8a/7329833/b72e15ab1b25/41598_2020_67214_Fig5_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/db8a/7329833/f629695a1134/41598_2020_67214_Fig1_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/db8a/7329833/a73d0ea259c2/41598_2020_67214_Fig2_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/db8a/7329833/8cac386754fc/41598_2020_67214_Fig3_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/db8a/7329833/5958e46b735c/41598_2020_67214_Fig4_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/db8a/7329833/b72e15ab1b25/41598_2020_67214_Fig5_HTML.jpg

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本文引用的文献

1
Grating-like nanostructures formed by the focused fs laser pulse in the volume of transparent dielectric.由聚焦飞秒激光脉冲在透明电介质体积内形成的类光栅纳米结构。
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Femtosecond response of polyatomic molecules to ultra-intense hard X-rays.
多原子分子对超强度硬 X 射线的飞秒响应。
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Revealing Three-Dimensional Structure of an Individual Colloidal Crystal Grain by Coherent X-Ray Diffractive Imaging.通过相干X射线衍射成像揭示单个胶体晶体颗粒的三维结构
Phys Rev Lett. 2016 Sep 23;117(13):138002. doi: 10.1103/PhysRevLett.117.138002. Epub 2016 Sep 22.
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X-ray laser-induced electron dynamics observed by femtosecond diffraction from nanocrystals of Buckminsterfullerene.X 射线激光诱导的电子动力学通过富勒烯纳米晶体的飞秒衍射观察到。
Sci Adv. 2016 Sep 9;2(9):e1601186. doi: 10.1126/sciadv.1601186. eCollection 2016 Sep.
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Transient Plasma Photonic Crystals for High-Power Lasers.用于高功率激光器的瞬态等离子体光子晶体
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Measurements of continuum lowering in solid-density plasmas created from elements and compounds.固体密度等离子体中连续体降低的测量,这些等离子体由元素和化合物产生。
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Nanosecond formation of diamond and lonsdaleite by shock compression of graphite.通过对石墨进行冲击压缩实现纳秒级金刚石和六方金刚石的形成。
Nat Commun. 2016 Mar 14;7:10970. doi: 10.1038/ncomms10970.
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Sci Rep. 2015 Jun 18;5:11089. doi: 10.1038/srep11089.
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The X-ray Pump-Probe instrument at the Linac Coherent Light Source.直线加速器相干光源处的X射线泵浦-探测仪。
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