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在阳极氧化TiO模板上制备的纳米多孔Co/Pd多层薄膜的磁性与磁阻特性的相关性

Correlation of magnetic and magnetoresistive properties of nanoporous Co/Pd thin multilayers fabricated on anodized TiO templates.

作者信息

Nguyen Thi Ngoc Anh, Kasiuk Julia, Wu Wen-Bin, Fedotova Julia, Przewoźnik Janusz, Kapusta Czesław, Kupreeva Olga, Lazarouk Serguei, Cao Thi Thanh Hai, Nguyen Thi Thanh Thuy, Dinh Hung Manh, Do Khanh Tung, Nguyen Thanh Huong, Vu Hong Ky, Vu Dinh Lam, Åkerman Johan

机构信息

Institute of Materials Science, Vietnam Academy of Science and Technology, 18 Hoang Quoc Viet, Cau Giay, Hanoi, Vietnam.

Vietnam Academy of Science and Technology, Graduate University of Science and Technology, 18 Hoang Quoc Viet, Cau Giay, Hanoi, Vietnam.

出版信息

Sci Rep. 2020 Jul 2;10(1):10838. doi: 10.1038/s41598-020-67677-0.

DOI:10.1038/s41598-020-67677-0
PMID:32616749
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC7331621/
Abstract

In this study, we consider a technological approach to obtain a high perpendicular magnetic anisotropy of the Co/Pd multilayers deposited on nanoporous TiO templates of different types of surface morphology. It is found that the use of templates with homogeneous and smoothed surface relief, formed on silicon wafers, ensures conservation of perpendicular anisotropy of the deposited films inherent in the continuous multilayers. Also, their magnetic hardening with doubling of the coercive field is observed. However, inhomogeneous magnetic ordering is revealed in the porous films due to the occurrence of magnetically soft regions near the pore edges and/or inside the pores. Modeling of the field dependences of magnetization and electrical resistance indicates that coherent rotation is the dominant mechanism of magnetization reversal in the porous system instead of the domain-wall motion typical of the continuous multilayers, while their magnetoresistance is determined by electron-magnon scattering, similarly to the continuous counterpart. The preservation of spin waves in the porous films indicates a high uniformity of the magnetic ordering in the fabricated porous systems due to a sufficiently regular pores array introduced into the films, despite the existence of soft-magnetic regions. The results are promising for the design and fabrication of future spintronic devices.

摘要

在本研究中,我们考虑一种技术方法,以获得沉积在具有不同表面形态类型的纳米多孔TiO模板上的Co/Pd多层膜的高垂直磁各向异性。结果发现,使用在硅片上形成的具有均匀且平滑表面起伏的模板,可确保沉积膜保留连续多层膜所固有的垂直各向异性。此外,还观察到其矫顽场加倍导致的磁硬化现象。然而,由于在孔边缘附近和/或孔内部出现磁软区域,在多孔膜中发现了不均匀的磁有序。对磁化强度和电阻的场依赖性进行建模表明,在多孔系统中,相干旋转是磁化反转的主导机制,而非连续多层膜典型的畴壁运动,同时,与连续多层膜类似,其磁电阻由电子-磁振子散射决定。尽管存在软磁区域,但由于在膜中引入了足够规则的孔阵列,多孔膜中自旋波的保留表明所制备的多孔系统中磁有序具有高度均匀性。这些结果对于未来自旋电子器件的设计和制造具有重要意义。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/ce08/7331621/44898b9053a9/41598_2020_67677_Fig6_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/ce08/7331621/c43aa3c5fbcc/41598_2020_67677_Fig1_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/ce08/7331621/54a39c036055/41598_2020_67677_Fig2_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/ce08/7331621/d452ea53ffc0/41598_2020_67677_Fig3_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/ce08/7331621/ec3798c75caa/41598_2020_67677_Fig4_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/ce08/7331621/cb0b987d78c8/41598_2020_67677_Fig5_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/ce08/7331621/44898b9053a9/41598_2020_67677_Fig6_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/ce08/7331621/c43aa3c5fbcc/41598_2020_67677_Fig1_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/ce08/7331621/54a39c036055/41598_2020_67677_Fig2_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/ce08/7331621/d452ea53ffc0/41598_2020_67677_Fig3_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/ce08/7331621/ec3798c75caa/41598_2020_67677_Fig4_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/ce08/7331621/cb0b987d78c8/41598_2020_67677_Fig5_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/ce08/7331621/44898b9053a9/41598_2020_67677_Fig6_HTML.jpg

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本文引用的文献

1
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Phys Chem Chem Phys. 2020 Feb 14;22(6):3661-3674. doi: 10.1039/c9cp05947d. Epub 2020 Jan 31.
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Anatomy of interfacial spin-orbit coupling in Co/Pd multilayers using X-ray magnetic circular dichroism and first-principles calculations.利用X射线磁性圆二色性和第一性原理计算研究Co/Pd多层膜中的界面自旋轨道耦合结构
Sci Rep. 2018 May 29;8(1):8303. doi: 10.1038/s41598-018-26195-w.
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Exchange Bias in the [CoO/Co/Pd] Antidot Large Area Arrays.
[CoO/Co/Pd] 反位错大面阵中的交换偏置。
ACS Appl Mater Interfaces. 2017 Sep 27;9(38):33250-33256. doi: 10.1021/acsami.7b07665. Epub 2017 Sep 18.
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