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定量源识别与两种不同土地利用类型下重金属的分配:两种受体模型 APCS-MLR 和 PMF 的比较。

Quantitative source identification and apportionment of heavy metals under two different land use types: comparison of two receptor models APCS-MLR and PMF.

机构信息

College of Life and Environmental Sciences, Minzu University of China, Beijing, 100081, China.

Guangxi Key Laboratory of Marine Disaster in the Beibu Gulf, Beibu Gulf University, Qinzhou, 535011, China.

出版信息

Environ Sci Pollut Res Int. 2020 Dec;27(34):42996-43010. doi: 10.1007/s11356-020-10234-z. Epub 2020 Jul 28.

DOI:10.1007/s11356-020-10234-z
PMID:32725567
Abstract

At present, many researchers are increasingly aware of the importance of using models to identify heavy metal (HM) pollution sources. However, on the performance and application of different source identification models to HMs under different land use types had been studied little. In this study, comparison of absolute principal component scores-multiple linear regression (APCS-MLR) and positive matrix factorization (PMF) models and their application characteristics in identifying pollution sources were carried out by using 11 HMs in Zhongwei City farmland and Shizuishan industrial park, Ningxia. The results indicated that HM pollution in farmland mainly came from pesticides, fertilizers, and deposition of the Yellow River, while the pollution in industrial park mainly originated from atmospheric deposition and various industrial productions. The APCS-MLR model had the problem of less identification sources and the difficulty to explain the complex pollution, while the PMF model not only identified more pollution sources, but also distinguished heavy metal-related sources for two different land use types and different industrial production conditions. It is of great significance the formulation of agricultural-related pesticides' and chemical fertilizers' rational use and various industrial production-related raw materials put in and emission control strategies.

摘要

目前,越来越多的研究人员意识到使用模型来识别重金属(HM)污染源的重要性。然而,对于不同土地利用类型下不同源识别模型对 HMs 的性能和应用,研究甚少。本研究通过对宁夏中卫市农田和石嘴山工业园区的 11 种重金属进行分析,比较了绝对主成分得分-多元线性回归(APCS-MLR)和正定矩阵因子分解(PMF)模型及其在识别污染源方面的应用特点。结果表明,农田重金属污染主要来源于农药、化肥和黄河沉积,而工业园区的污染主要来源于大气沉降和各种工业生产。APCS-MLR 模型存在识别源较少、难以解释复杂污染的问题,而 PMF 模型不仅能识别更多的污染源,还能区分两种不同土地利用类型和不同工业生产条件下与重金属相关的污染源。这对于制定与农业相关的农药和化肥合理使用以及各种工业生产相关原材料投入和排放控制策略具有重要意义。

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