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流场中空化的发光与化学发光的对比研究及其羟基自由基生成的定量测定。

Comparative study of luminescence and chemiluminescence in hydrodynamic cavitating flows and quantitative determination of hydroxyl radicals production.

机构信息

Laboratoire des Ecoulements Géophysiques et Industriels, Univ. Grenoble Alpes, CNRS, 38000 Grenoble, France.

Laboratoire des Ecoulements Géophysiques et Industriels, Univ. Grenoble Alpes, CNRS, 38000 Grenoble, France.

出版信息

Ultrason Sonochem. 2021 Jan;70:105277. doi: 10.1016/j.ultsonch.2020.105277. Epub 2020 Jul 27.

DOI:10.1016/j.ultsonch.2020.105277
PMID:32750656
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC7786554/
Abstract

Luminescence and chemiluminescence have been experimentally investigated in hydrodynamic cavitating flows. By using dedicated microdevices inserted inside a light tight box, photons counting has been made possible. Luminescence has been investigated with deionized water as the working fluid; chemiluminescence has resulted from cavitating alkaline luminol solutions, and has been correlated to hydroxyl radicals formation. For the first time, luminescent and chemiluminescent phenomena have been considered together on the same devices submitted to similar cavitating flow regimes. Degassed solutions enhance the luminescence and also the hydroxyl radical yield. Due to the small sizes of the channels, the lifetimes of the collapsing bubbles correspond to pseudo frequencies matching the range of optimal frequencies used in sonochemistry. New perspectives for the study of hydrodynamic cavitation as an advanced oxidation process are suggested.

摘要

已在流体动力学空化流中对发光和化学发光进行了实验研究。通过使用插入在不透光盒子内的专用微器件，实现了光子计数。使用去离子水作为工作流体研究了发光；化学发光来自空化碱性鲁米诺溶液，并与羟基自由基的形成相关联。首次在相同的装置上同时考虑了发光和化学发光现象，这些装置经历了类似的空化流状态。除气溶液增强了发光和羟基自由基的产率。由于通道尺寸较小，崩溃气泡的寿命与匹配声化学中使用的最佳频率范围的拟频率相对应。建议将流体动力学空化作为一种高级氧化工艺进行研究的新视角。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a5cb/7786554/401c56dc24c7/gr9.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a5cb/7786554/2dbd2bddc297/gr1.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a5cb/7786554/ed25e5bce3da/gr2.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a5cb/7786554/c763d1934b8c/gr3.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a5cb/7786554/33d591bca165/gr4.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a5cb/7786554/df7ce829fdc2/gr5.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a5cb/7786554/373bfadcfc80/gr6.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a5cb/7786554/8628ffc2d83a/gr7.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a5cb/7786554/1b63c249a63d/gr8.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a5cb/7786554/401c56dc24c7/gr9.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a5cb/7786554/2dbd2bddc297/gr1.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a5cb/7786554/ed25e5bce3da/gr2.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a5cb/7786554/c763d1934b8c/gr3.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a5cb/7786554/33d591bca165/gr4.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a5cb/7786554/df7ce829fdc2/gr5.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a5cb/7786554/373bfadcfc80/gr6.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a5cb/7786554/8628ffc2d83a/gr7.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a5cb/7786554/1b63c249a63d/gr8.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a5cb/7786554/401c56dc24c7/gr9.jpg

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本文引用的文献

1
The Chemical History of a Bubble.一个气泡的化学历程。
Acc Chem Res. 2018 Sep 18;51(9):2169-2178. doi: 10.1021/acs.accounts.8b00088. Epub 2018 May 17.
2
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Ultrason Sonochem. 2018 May;43:175-183. doi: 10.1016/j.ultsonch.2018.01.004. Epub 2018 Jan 4.
3
Experimental evidence of temperature gradients in cavitating microflows seeded with thermosensitive nanoprobes.
Phys Rev E Stat Nonlin Soft Matter Phys. 2013 Oct;88(4):043016. doi: 10.1103/PhysRevE.88.043016. Epub 2013 Oct 31.
4
Dissolved gas and ultrasonic cavitation--a review.溶解气体与超声空化——综述。
Ultrason Sonochem. 2013 Jan;20(1):1-11. doi: 10.1016/j.ultsonch.2012.04.013. Epub 2012 May 24.
5
A theoretical study of hydrodynamic cavitation.水力空化的理论研究。
Ultrason Sonochem. 2008 Mar;15(3):203-11. doi: 10.1016/j.ultsonch.2007.03.007. Epub 2007 Apr 2.
6
Application of salicylic acid dosimetry to evaluate hydrodynamic cavitation as an advanced oxidation process.应用水杨酸剂量测定法评估作为一种高级氧化工艺的水力空化作用。
Ultrason Sonochem. 2007 Mar;14(3):343-9. doi: 10.1016/j.ultsonch.2006.06.007. Epub 2006 Oct 5.
7
Plasma formation and temperature measurement during single-bubble cavitation.单泡空化过程中的等离子体形成与温度测量。
Nature. 2005 Mar 3;434(7029):52-5. doi: 10.1038/nature03361.
8
Single-bubble sonochemiluminescence in aqueous luminol solutions.鲁米诺水溶液中的单泡声致化学发光
J Am Chem Soc. 2002 Sep 4;124(35):10250-1. doi: 10.1021/ja0258475.
9
The energy efficiency of formation of photons, radicals and ions during single-bubble cavitation.单泡空化过程中光子、自由基和离子形成的能量效率。
Nature. 2002 Jul 25;418(6896):394-7. doi: 10.1038/nature00895.
10
Ultrasonic waste-water treatment: incidence of ultrasonic frequency on the rate of phenol and carbon tetrachloride degradation.
Ultrason Sonochem. 1997 Oct;4(4):295-300. doi: 10.1016/s1350-4177(97)00036-9.