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泰国受城市污水排放影响的水生环境和沿海水中的新兴污染物:生态风险视角。

Emerging contaminants in aquatic environments and coastal waters affected by urban wastewater discharge in Thailand: An ecological risk perspective.

机构信息

State Key Laboratory of Organic Geochemistry, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou, 510640, China; SCNU Environmental Research Institute, Guangdong Provincial Key Laboratory of Chemical Pollution and Environmental Safety & MOE Key Laboratory of Environmental Theoretical Chemistry, South China Normal University, Guangzhou, 510006, China; School of Environment, South China Normal University, University Town, Guangzho, 510006, China; University of Chinese Academy of Sciences, Beijing, 100049, China.

SCNU Environmental Research Institute, Guangdong Provincial Key Laboratory of Chemical Pollution and Environmental Safety & MOE Key Laboratory of Environmental Theoretical Chemistry, South China Normal University, Guangzhou, 510006, China; School of Environment, South China Normal University, University Town, Guangzho, 510006, China.

出版信息

Ecotoxicol Environ Saf. 2020 Nov;204:110952. doi: 10.1016/j.ecoenv.2020.110952. Epub 2020 Aug 12.

Abstract

Emerging contaminants such as synthetic musks and UV-filters as ingredients personal care products were widely used in human daily life in Thailand. The occurrence and fate of four synthetic musks and nine UV-filters were investigated in eight full-scale sewage treatment plants (STPs) and their receiving aquatic environments in Bangkok and Pattaya, Thailand. All target compounds were detected in every single sample from STPs and surface water with magnitude from ng/L to μg/L. HHCB-lactone and HMS were found as the predominant musk and UV filter in influent and effluent of STPs, respectively. HHCB-lactone was also found with the highest concentration up to 79501 ng/g (dw) in the sludge. Low removal efficiency range from -37% (HHCB-lactone) to 58% (AHTN) were found for four musks in the STPs. The total emission of Σmusks and ΣUV-filters were estimated to be up to 16.7 mg/person/day and 0.28 mg/person/day by the STPs. Three synthetic musks and seven UV-filters were detected in fish from the receiving river. Concentration and emission of musks and UV filters found in this study from Thailand were much higher than those reported in many other countries worldwide. The preliminary ecological risk assessment showed that Musk xylene, 4-MBC and OC may pose high risk to aquatic organisms in the riverine and estuarine environment in Thailand.

摘要

新兴污染物,如合成麝香和紫外线滤光剂作为个人护理产品的成分,在泰国的人类日常生活中被广泛使用。本研究调查了 8 座全规模污水处理厂(STP)及其接收的水生环境中 4 种合成麝香和 9 种紫外线滤光剂的出现和归宿。所有目标化合物均在曼谷和芭堤雅的 STP 和地表水的每一个单独样本中被检出,浓度范围为 ng/L 至 μg/L。HHCB-内酯和 HMS 分别是 STP 进、出水的主要麝香和紫外线滤光剂。HHCB-内酯在污泥中的浓度最高,达 79501ng/g(干重)。在 STP 中,4 种麝香的去除效率范围为 -37%(HHCB-内酯)至 58%(AHTN)。通过 STP 估算,Σ麝香和 Σ紫外线滤光剂的总排放量分别高达 16.7 毫克/人/天和 0.28 毫克/人/天。在河流中的鱼类中检测到三种合成麝香和七种紫外线滤光剂。本研究中在泰国发现的麝香和紫外线滤光剂的浓度和排放量远高于全球许多其他国家的报告。初步生态风险评估显示,二甲苯麝香、4-MBC 和 OC 可能对泰国河流和河口环境中的水生生物构成高风险。

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