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低密度互连纳米线网络中的三维纳米磁性

3D Nanomagnetism in Low Density Interconnected Nanowire Networks.

作者信息

Burks Edward C, Gilbert Dustin A, Murray Peyton D, Flores Chad, Felter Thomas E, Charnvanichborikarn Supakit, Kucheyev Sergei O, Colvin Jeffrey D, Yin Gen, Liu Kai

机构信息

Physics Department, University of California, Davis, California 95618, United States.

Department of Materials Science and Engineering, University of Tennessee, Knoxville, Tennessee 37996, United States.

出版信息

Nano Lett. 2021 Jan 13;21(1):716-722. doi: 10.1021/acs.nanolett.0c04366. Epub 2020 Dec 10.

Abstract

Free-standing, interconnected metallic nanowire networks with densities as low as 40 mg/cm have been achieved over centimeter-scale areas, using electrodeposition into polycarbonate membranes that have been ion-tracked at multiple angles. Networks of interconnected magnetic nanowires further provide an exciting platform to explore 3-dimensional nanomagnetism, where their structure, topology, and frustration may be used as additional degrees of freedom to tailor the materials properties. New magnetization reversal mechanisms in cobalt networks are captured by the first-order reversal curve method, which demonstrate the evolution from strong demagnetizing dipolar interactions to intersection-mediated domain wall pinning and propagation, and eventually to shape-anisotropy dominated magnetization reversal. These findings open up new possibilities for 3-dimensional integrated magnetic devices for memory, complex computation, and neuromorphics.

摘要

通过将金属电沉积到经多角度离子径迹蚀刻的聚碳酸酯膜中,已在厘米级面积上实现了密度低至40 mg/cm的独立、相互连接的金属纳米线网络。相互连接的磁性纳米线网络进一步提供了一个令人兴奋的平台,用于探索三维纳米磁性,在这个平台中,它们的结构、拓扑结构和阻挫现象可作为额外的自由度来调整材料特性。钴网络中的新磁化反转机制通过一阶反转曲线法得以捕捉,该方法证明了从强退磁偶极相互作用到交叉介导的畴壁钉扎和传播,最终到形状各向异性主导的磁化反转的演变过程。这些发现为用于存储器、复杂计算和神经形态学的三维集成磁器件开辟了新的可能性。

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