Zhang Qing, Shang Qiuyu, Su Rui, Do T Thu Ha, Xiong Qihua
School of Materials Science and Engineering, College of Engineering, Peking University, Beijing 100871, China.
Research Center for Wide Gap Semiconductor, Peking University, Beijing 100871, China.
Nano Lett. 2021 Mar 10;21(5):1903-1914. doi: 10.1021/acs.nanolett.0c03593. Epub 2021 Jan 12.
Solution-processable semiconductor lasers have been a long-standing challenge for next-generation displays, light sources, and communication technologies. Metal halide perovskites, which combine the advantages of inorganic and organic semiconductors, have recently emerged not only as excellent candidates for solution-processable lasers but also as potential complementary gain materials for filling the "green gap" and supplement industrial nanolasers based on classic II-VI/III-V semiconductors. Numerous perovskite lasers have been developed successfully with superior performance in terms of cost-effectiveness, low threshold, high coherence, and multicolor tunability. This mini review surveys the development, current status, and perspectives of perovskite lasers, categorized into thin film lasers, nanocrystals lasers, microlasers, and device concepts including polariton and bound-in-continuum lasers with a focus on material fundamentals, cavity design, and low-threshold devices in addition to critical issues such as mass fabrication and applications.
可溶液加工的半导体激光器一直是下一代显示器、光源和通信技术面临的长期挑战。金属卤化物钙钛矿结合了无机和有机半导体的优点,最近不仅成为可溶液加工激光器的优秀候选材料,还成为填补“绿色差距”的潜在互补增益材料,并补充基于经典II-VI/III-V半导体的工业纳米激光器。众多钙钛矿激光器已成功开发,在成本效益、低阈值、高相干性和多色可调性方面具有卓越性能。本综述调查了钙钛矿激光器的发展、现状和前景,分为薄膜激光器、纳米晶体激光器、微激光器以及包括极化激元激光器和连续束缚态激光器在内的器件概念,重点关注材料基础、腔设计和低阈值器件,此外还涉及大规模制造和应用等关键问题。