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近年来卤化铅钙钛矿中强激子-光子耦合的进展。

Recent Progress of Strong Exciton-Photon Coupling in Lead Halide Perovskites.

机构信息

Division of Nanophotonics, CAS Key Laboratory of Standardization and Measurement for Nanotechnology, CAS Center for Excellence in Nanoscience, National Center for Nanoscience and Technology, Beijing, 100190, P. R. China.

University of Chinese Academy of Sciences, 19 A Yuquan Rd, Shijingshan District, Beijing, 100049, P. R. China.

出版信息

Adv Mater. 2019 Nov;31(45):e1804894. doi: 10.1002/adma.201804894. Epub 2018 Nov 6.

Abstract

The semiconductor exciton-polariton, arising from the strong coupling between excitons and confined cavity photon modes, is not only of fundamental importance in macroscopic quantum effects but also has wide application prospects in ultralow-threshold polariton lasers, slowing-light devices, and quantum light sources. Very recently, metallic halide perovskites have been considered as a great candidate for exciton-polariton devices owing to their low-cost fabrication, large exciton oscillator strength, and binding energy. Herein, the latest progress in exciton-polaritons and polariton lasers of perovskites are reviewed. Polaritons in planar and nanowires Fabry-Pérot microcavities are discussed with particular reference to material and photophysics. Finally, a perspective on the remaining challenges in perovskite polaritons research is given.

摘要

半导体激子-极化激元,源于激子和受限腔光子模式之间的强耦合,不仅在宏观量子效应中具有重要意义,而且在超低阈值极化激元激光器、光缓变器件和量子光源中也具有广泛的应用前景。最近,金属卤化物钙钛矿由于其低成本的制造工艺、大的激子振子强度和束缚能,被认为是激子-极化激元器件的理想候选材料。本文综述了钙钛矿中激子-极化激元和极化激元激光的最新进展。特别参考了材料和光物理方面,讨论了平面和纳米线法布里-珀罗微腔中的极化激元。最后,对钙钛矿极化激元研究中尚存的挑战进行了展望。

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