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用于先进锌离子水系电池的阴极材料的微观结构工程

Microstructural Engineering of Cathode Materials for Advanced Zinc-Ion Aqueous Batteries.

作者信息

Pam Mei Er, Yan Dong, Yu Juezhi, Fang Daliang, Guo Lu, Li Xue Liang, Li Tian Chen, Lu Xunyu, Ang Lay Kee, Amal Rose, Han Zhaojun, Yang Hui Ying

机构信息

Pillar of Engineering Product Development Singapore University of Technology and Design 8 Somapah Road Singapore 487372 Singapore.

Science and Math Cluster Singapore University of Technology and Design (SUTD) 8 Somapah Road Singapore 487372 Singapore.

出版信息

Adv Sci (Weinh). 2020 Nov 19;8(1):2002722. doi: 10.1002/advs.202002722. eCollection 2020 Jan.

DOI:10.1002/advs.202002722
PMID:33437582
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC7788579/
Abstract

Zinc-ion batteries (ZIBs) have attracted intensive attention due to the low cost, high safety, and abundant resources. However, up to date, challenges still exist in searching for cathode materials with high working potential, excellent electrochemical activity, and good structural stability. To address these challenges, microstructure engineering has been widely investigated to modulate the physical properties of cathode materials, and thus boosts the electrochemical performances of ZIBs. Here, the recent research efforts on the microstructural engineering of various ZIB cathode materials are mainly focused upon, including composition and crystal structure selection, crystal defect engineering, interlayer engineering, and morphology design. The dependency of cathode performance on aqueous electrolyte for ZIB is further discussed. Finally, future perspectives and challenges on microstructure engineering of cathode materials for ZIBs are provided. It is aimed to provide a deep understanding of the microstructure engineering effect on Zn storage performance.

摘要

锌离子电池（ZIBs）因其成本低、安全性高和资源丰富而备受关注。然而，迄今为止，在寻找具有高工作电位、优异电化学活性和良好结构稳定性的阴极材料方面仍存在挑战。为应对这些挑战，人们广泛研究了微观结构工程以调节阴极材料的物理性能，从而提高锌离子电池的电化学性能。在此，主要聚焦于各种锌离子电池阴极材料微观结构工程的最新研究成果，包括成分和晶体结构选择、晶体缺陷工程、层间工程和形貌设计。进一步讨论了锌离子电池阴极性能对水性电解质的依赖性。最后，给出了锌离子电池阴极材料微观结构工程的未来展望和挑战。旨在深入理解微观结构工程对锌存储性能的影响。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/3c50/7788579/1c0a6609ef77/ADVS-8-2002722-g010.jpg
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